Metal-Oxide-Based Microjets for the Simultaneous Removal of Organic Pollutants and Heavy Metals

Water contamination from industrial and anthropogenic activities is nowadays a major issue in many countries worldwide. To address this problem, efficient water treatment technologies are required. Recent efforts have focused on the development of self-propelled micromotors that provide enhanced mic...

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Veröffentlicht in:ACS applied materials & interfaces 2018-06, Vol.10 (24), p.20478-20486
Hauptverfasser: Villa, Katherine, Parmar, Jemish, Vilela, Diana, Sánchez, Samuel
Format: Artikel
Sprache:eng
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Zusammenfassung:Water contamination from industrial and anthropogenic activities is nowadays a major issue in many countries worldwide. To address this problem, efficient water treatment technologies are required. Recent efforts have focused on the development of self-propelled micromotors that provide enhanced micromixing and mass transfer by the transportation of reactive species, resulting in higher decontamination rates. However, a real application of these micromotors is still limited due to the high cost associated to their fabrication process. Here, we present Fe2O3-decorated SiO2/MnO2 microjets for the simultaneous removal of industrial organic pollutants and heavy metals present in wastewater. These microjets were synthesized by low-cost and scalable methods. They exhibit an average speed of 485 ± 32 μm s–1 (∼28 body length per s) at 7% H2O2, which is the highest reported for MnO2-based tubular micromotors. Furthermore, the photocatalytic and adsorbent properties of the microjets enable the efficient degradation of organic pollutants, such as tetracycline and rhodamine B under visible light irradiation, as well as the removal of heavy metal ions, such as Cd2+ and Pb2+.
ISSN:1944-8244
1944-8252
DOI:10.1021/acsami.8b04353