Review of brown carbon aerosols: Recent progress and perspectives

•Emission factors of brown carbon from different emission sources are summarized.•Including the effects of photochemical brown carbon can improve models' skills.•Key factors influencing the radiative forcing of brown carbon were identified. [Display omitted] Brown carbon (BrC), a carbonaceous a...

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Veröffentlicht in:The Science of the total environment 2018-09, Vol.634, p.1475-1485
Hauptverfasser: Yan, Juping, Wang, Xiaoping, Gong, Ping, Wang, Chuanfei, Cong, Zhiyuan
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Sprache:eng
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Zusammenfassung:•Emission factors of brown carbon from different emission sources are summarized.•Including the effects of photochemical brown carbon can improve models' skills.•Key factors influencing the radiative forcing of brown carbon were identified. [Display omitted] Brown carbon (BrC), a carbonaceous aerosol which absorbs solar radiation over a broad range of wavelengths, is beginning to be seen as an important contributor to global warming. BrC absorbs both inorganic and organic pollutants, leading to serious effects on human health. We review the fundamental features of BrC, including its sources, chemical composition, optical properties and radiative forcing effects. We detail the importance of including photochemical processes related to BrC in the GEOS-Chem transport model for the estimation of aerosol radiative forcing. Calculation methods for BrC emission factors are examined, including the problems and limitations of current measurement methods. We provide some insight into existing publications and recommend areas for future research, such as further investigations into the reaction mechanisms of the aging of secondary BrC, calculations of the emission factors for BrC from different sources, the absorption of large and long-lived BrC molecules and the construction of an enhanced model for the simulation of radiative forcing. This review will improve our understanding of the climatic and environmental effects of BrC.
ISSN:0048-9697
1879-1026
DOI:10.1016/j.scitotenv.2018.04.083