Activity statistics in a colloidal glass former: Experimental evidence for a dynamical transition

In a dense colloidal suspension at a volume fraction below the glass transition, we follow the trajectories of an assembly of tracers over a large time window. We define a local activity, which quantifies the local tendency of the system to rearrange. We determine the statistics of the time integrat...

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Veröffentlicht in:The Journal of chemical physics 2018-04, Vol.148 (16), p.164502-164502
Hauptverfasser: Abou, Bérengère, Colin, Rémy, Lecomte, Vivien, Pitard, Estelle, van Wijland, Frédéric
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Sprache:eng
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Zusammenfassung:In a dense colloidal suspension at a volume fraction below the glass transition, we follow the trajectories of an assembly of tracers over a large time window. We define a local activity, which quantifies the local tendency of the system to rearrange. We determine the statistics of the time integrated activity, and we argue that it develops a low activity tail that comes together with the onset of glassy-like behavior and heterogeneous dynamics. These rare events may be interpreted as the reflection of an underlying dynamic phase transition.
ISSN:0021-9606
1089-7690
DOI:10.1063/1.5006924