Evaluating multimedia/multipathway model intake fraction estimates using POP emission and monitoring data

This paper presents a structured evaluation of a novel multimedia chemical fate and multi-pathway human exposure model for Western Europe, IMPACT 2002, using data for PCDD/F congeners. PCDD/F congeners provide an illustration of the potential use of POPs (Persistent Organic Pollutant) data for the e...

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Veröffentlicht in:Environmental pollution (1987) 2004-01, Vol.128 (1), p.263-277
Hauptverfasser: Margni, M., Pennington, D.W., Amman, C., Jolliet, O.
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container_title Environmental pollution (1987)
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creator Margni, M.
Pennington, D.W.
Amman, C.
Jolliet, O.
description This paper presents a structured evaluation of a novel multimedia chemical fate and multi-pathway human exposure model for Western Europe, IMPACT 2002, using data for PCDD/F congeners. PCDD/F congeners provide an illustration of the potential use of POPs (Persistent Organic Pollutant) data for the evaluation of such models. Based on available emission estimates, model predictions with and without spatial resolution are evaluated at three different stages against monitored data: at environmental contamination levels, food exposure concentration, and in terms of human intake fractions ( iF): the fraction of an emission that is taken in by the population. The iF is ∼3.5·10 −3 for emissions of dioxin in Western Europe. This iF compares well to the traditional non-spatial multi-media/-pathway model predictions of 3.9·10 −3 for the same region and to 2·10 −3 for the USA. Approximately 95% of the intake from Western European emissions occurs within the same region, 5% being transferred out of the region in terms of food contaminants and atmospheric advective transport. The fraction of PCDD/F Emission which transfers to the human population is assessed for Europe using a novel approach.
doi_str_mv 10.1016/j.envpol.2003.08.036
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subjects Air Pollution
Air. Soil. Water. Waste. Feeding
Animal, plant and microbial ecology
Applied ecology
Applied sciences
Atmospheric pollution
Biological and medical sciences
Data Collection
Dioxin
Earth sciences
Earth, ocean, space
Ecotoxicology, biological effects of pollution
Engineering and environment geology. Geothermics
Environment. Living conditions
Environmental Exposure
Environmental Monitoring - methods
Environmental Pollutants - toxicity
Environmental Pollution
Europe
Exact sciences and technology
Food Contamination
Fundamental and applied biological sciences. Psychology
General aspects
Intake fraction
Medical sciences
Model evaluation
Models, Theoretical
Multi-exposure-pathways
Multimedia models
Organic Chemicals - toxicity
PCDD
PCDF
persistent organic pollutants
Pollutants physicochemistry study: properties, effects, reactions, transport and distribution
Pollution
Pollution, environment geology
Public health. Hygiene
Public health. Hygiene-occupational medicine
Soil Pollutants
Time Factors
title Evaluating multimedia/multipathway model intake fraction estimates using POP emission and monitoring data
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