A parametric study of CO sub(2)/N sub(2) gas separation membrane processes for post-combustion capture

Capture of CO sub(2) from flue gases produced by the combustion of fossil fuels and biomass in air is referred to as post-combustion capture. Chemisorbent processes are considered to be the most feasible method and are already at an advanced stage of development, but gas separation membranes are att...

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Veröffentlicht in:Journal of membrane science 2008-11, Vol.325 (1), p.284-294
Hauptverfasser: Zhao, Li, Riensche, Ernst, Menzer, Reinhard, Blum, Ludger, Stolten, Detlef
Format: Artikel
Sprache:eng
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Zusammenfassung:Capture of CO sub(2) from flue gases produced by the combustion of fossil fuels and biomass in air is referred to as post-combustion capture. Chemisorbent processes are considered to be the most feasible method and are already at an advanced stage of development, but gas separation membranes are attracting more and more attention as a possible alternative. This paper describes a detailed parametric study of mass and energy balances for a simulated single membrane process. Typical operating conditions (CO sub(2) concentration in the flue gas, pressure and temperature, etc.) together with the influence of the membrane quality (permeability, selectivity) and membrane area on membrane performance (CO sub(2) separation degree and CO sub(2) purity) are simulated over a wide range of parameters.
ISSN:0376-7388
DOI:10.1016/j.memsci.2008.07.058