Stable Hematite Nanosheet Photoanodes for Enhanced Photoelectrochemical Water Splitting

A vertically grown hematite nanosheet film modified with Ag nanoparticles (NPs) and Co–Pi cocatalyst exhibits a remarkably high photocurrent density of 4.68 mA cm−2 at 1.23 V versus RHE. The Ag NPs leads to significantly improved light harvesting and better charge transfer, while the Co–Pi facilitat...

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Veröffentlicht in:Advanced materials (Weinheim) 2016-08, Vol.28 (30), p.6405-6410
Hauptverfasser: Peerakiatkhajohn, Piangjai, Yun, Jung-Ho, Chen, Hongjun, Lyu, Miaoqiang, Butburee, Teera, Wang, Lianzhou
Format: Artikel
Sprache:eng
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Zusammenfassung:A vertically grown hematite nanosheet film modified with Ag nanoparticles (NPs) and Co–Pi cocatalyst exhibits a remarkably high photocurrent density of 4.68 mA cm−2 at 1.23 V versus RHE. The Ag NPs leads to significantly improved light harvesting and better charge transfer, while the Co–Pi facilitates a highly stable oxygen evolution process. This photoelectrode design provides more efficient photoelectrochemical systems for solar‐energy conversion.
ISSN:0935-9648
1521-4095
DOI:10.1002/adma.201601525