Complex Field-Induced States in Linarite PbCuSO sub(4)(OH) sub(2) with a Variety of High-Order Exotic Spin-Density Wave States

Low-temperature neutron diffraction and NMR studies of field-induced phases in linarite are presented for magnetic fields H || b axis. A two-step spin-flop transition is observed, as well as a transition transforming a helical magnetic ground state into an unusual magnetic phase with sine-wave-modul...

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Veröffentlicht in:Physical review letters 2016-01, Vol.116 (4)
Hauptverfasser: Willenberg, B, Schapers, M, Wolter, A U B, Drechsler, S-L, Reehuis, M, Hoffmann, J-U, Buchner, B, Studer, A J, Rule, K C, Ouladdiaf, B, Sullow, S, Nishimoto, S
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Sprache:eng
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Zusammenfassung:Low-temperature neutron diffraction and NMR studies of field-induced phases in linarite are presented for magnetic fields H || b axis. A two-step spin-flop transition is observed, as well as a transition transforming a helical magnetic ground state into an unusual magnetic phase with sine-wave-modulated moments ||H. An effective J sub(1) super(~)-J sub(2 ) super(~) single-chain model with a magnetization-dependent frustration ratio alpha sub(eff) = J sub(2)/J sub(1) is proposed. The latter is governed by skew interchain couplings and shifted to the vicinity of the ferromagnetic critical point. It explains qualitatively the observation of a rich variety of exotic longitudinal collinear spin-density wave, SDW sub(p), states (9 > or = p > or = 2).
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.116.047202