Anomalous Fano Profiles in External Fields

We show that the external control of Fano resonances in general leads to complex Fano q parameters. Fano line shapes of photoelectron and transient absorption spectra in the presence of an infrared control field are investigated. Computed transient absorption spectra are compared with a model propos...

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Veröffentlicht in:Physical review letters 2015-12, Vol.115 (24), p.243001-243001, Article 243001
Hauptverfasser: Zielinski, Alejandro, Majety, Vinay Pramod, Nagele, Stefan, Pazourek, Renate, Burgdörfer, Joachim, Scrinzi, Armin
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Sprache:eng
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Zusammenfassung:We show that the external control of Fano resonances in general leads to complex Fano q parameters. Fano line shapes of photoelectron and transient absorption spectra in the presence of an infrared control field are investigated. Computed transient absorption spectra are compared with a model proposed for a recent experiment [C. Ott et al., Science 340, 716 (2013)]. Control mechanisms for photoelectron spectra are exposed: control pulses applied during excitation modify the line shapes by momentum boosts of the continuum electrons. Pulses arriving after excitation generate interference fringes due to infrared two-photon transitions.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.115.243001