Signatures of molecular orbital structure in lateral electron momentum distributions from strong-field ionization
Strong-field ionization of aligned diatomic and polyatomic molecules such as O2, N2, C2H4, and others in circularly polarized laser fields is investigated theoretically. By calculating the emission-angle-resolved lateral width of the momentum distribution perpendicular to the polarization plane, we...
Gespeichert in:
| Veröffentlicht in: | Physical review letters 2015-03, Vol.114 (10), p.103004-103004, Article 103004 |
|---|---|
| Hauptverfasser: | , , |
| Format: | Artikel |
| Sprache: | eng |
| Schlagworte: | |
| Online-Zugang: | Volltext |
| Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
| container_end_page | 103004 |
|---|---|
| container_issue | 10 |
| container_start_page | 103004 |
| container_title | Physical review letters |
| container_volume | 114 |
| creator | Petersen, Ingo Henkel, Jost Lein, Manfred |
| description | Strong-field ionization of aligned diatomic and polyatomic molecules such as O2, N2, C2H4, and others in circularly polarized laser fields is investigated theoretically. By calculating the emission-angle-resolved lateral width of the momentum distribution perpendicular to the polarization plane, we show that nodal planes in molecular orbitals are directly imprinted on the angular dependence of the width. We demonstrate that orbital symmetries can be distinguished with the information obtained by observing the lateral width in addition to the angular distributions. |
| doi_str_mv | 10.1103/physrevlett.114.103004 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1786221529</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1667965926</sourcerecordid><originalsourceid>FETCH-LOGICAL-c511t-a91e6202df28d84ec7a7138fe677977863171ab45a27ae34c0c9be632cc52d143</originalsourceid><addsrcrecordid>eNqFkctKxTAQhoMoery8gmTppppJ26RZiniDA4qXdUnTqUbS5pikgj69ORx16yrwzf9PYD5CjoGdArDybPX6GQN-OEwpg-o0M8aqLbIAJlUhM9omC8ZKKBRjco_sx_jGGAMuml2yx-sGasXVgrw_2pdJpzlgpH6go3doZqcD9aGzSTsaU5jNek7tRJ1OGDLEnErBTzk_4pTmkfY2B203J-unSIfgx3XTTy_FYNH1NGP7pdfTQ7IzaBfx6Oc9IM9Xl08XN8Xy7vr24nxZmBogFVoBCs54P_Cmbyo0UksomwGFlErKRpQgQXdVrbnUWFaGGdWhKLkxNe-hKg_IyWbvKvj3GWNqRxsNOqcn9HNsIe_gHGqu_o8KIZXIBxM5KjZRE3zMBoZ2Feyow2cLrF2bae-zmQf8WGYzGVTtxkwuHv_8MXcj9n-1XxXlN_EQj9A</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1667965926</pqid></control><display><type>article</type><title>Signatures of molecular orbital structure in lateral electron momentum distributions from strong-field ionization</title><source>American Physical Society Journals</source><creator>Petersen, Ingo ; Henkel, Jost ; Lein, Manfred</creator><creatorcontrib>Petersen, Ingo ; Henkel, Jost ; Lein, Manfred</creatorcontrib><description>Strong-field ionization of aligned diatomic and polyatomic molecules such as O2, N2, C2H4, and others in circularly polarized laser fields is investigated theoretically. By calculating the emission-angle-resolved lateral width of the momentum distribution perpendicular to the polarization plane, we show that nodal planes in molecular orbitals are directly imprinted on the angular dependence of the width. We demonstrate that orbital symmetries can be distinguished with the information obtained by observing the lateral width in addition to the angular distributions.</description><identifier>ISSN: 0031-9007</identifier><identifier>EISSN: 1079-7114</identifier><identifier>DOI: 10.1103/physrevlett.114.103004</identifier><identifier>PMID: 25815929</identifier><language>eng</language><publisher>United States</publisher><subject>Angular distribution ; Angular momentum ; Ionization ; Lasers ; Mathematical analysis ; Molecular orbitals ; Planes ; Signatures</subject><ispartof>Physical review letters, 2015-03, Vol.114 (10), p.103004-103004, Article 103004</ispartof><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c511t-a91e6202df28d84ec7a7138fe677977863171ab45a27ae34c0c9be632cc52d143</citedby><cites>FETCH-LOGICAL-c511t-a91e6202df28d84ec7a7138fe677977863171ab45a27ae34c0c9be632cc52d143</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,2863,2864,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25815929$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Petersen, Ingo</creatorcontrib><creatorcontrib>Henkel, Jost</creatorcontrib><creatorcontrib>Lein, Manfred</creatorcontrib><title>Signatures of molecular orbital structure in lateral electron momentum distributions from strong-field ionization</title><title>Physical review letters</title><addtitle>Phys Rev Lett</addtitle><description>Strong-field ionization of aligned diatomic and polyatomic molecules such as O2, N2, C2H4, and others in circularly polarized laser fields is investigated theoretically. By calculating the emission-angle-resolved lateral width of the momentum distribution perpendicular to the polarization plane, we show that nodal planes in molecular orbitals are directly imprinted on the angular dependence of the width. We demonstrate that orbital symmetries can be distinguished with the information obtained by observing the lateral width in addition to the angular distributions.</description><subject>Angular distribution</subject><subject>Angular momentum</subject><subject>Ionization</subject><subject>Lasers</subject><subject>Mathematical analysis</subject><subject>Molecular orbitals</subject><subject>Planes</subject><subject>Signatures</subject><issn>0031-9007</issn><issn>1079-7114</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><recordid>eNqFkctKxTAQhoMoery8gmTppppJ26RZiniDA4qXdUnTqUbS5pikgj69ORx16yrwzf9PYD5CjoGdArDybPX6GQN-OEwpg-o0M8aqLbIAJlUhM9omC8ZKKBRjco_sx_jGGAMuml2yx-sGasXVgrw_2pdJpzlgpH6go3doZqcD9aGzSTsaU5jNek7tRJ1OGDLEnErBTzk_4pTmkfY2B203J-unSIfgx3XTTy_FYNH1NGP7pdfTQ7IzaBfx6Oc9IM9Xl08XN8Xy7vr24nxZmBogFVoBCs54P_Cmbyo0UksomwGFlErKRpQgQXdVrbnUWFaGGdWhKLkxNe-hKg_IyWbvKvj3GWNqRxsNOqcn9HNsIe_gHGqu_o8KIZXIBxM5KjZRE3zMBoZ2Feyow2cLrF2bae-zmQf8WGYzGVTtxkwuHv_8MXcj9n-1XxXlN_EQj9A</recordid><startdate>20150313</startdate><enddate>20150313</enddate><creator>Petersen, Ingo</creator><creator>Henkel, Jost</creator><creator>Lein, Manfred</creator><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7U5</scope><scope>8FD</scope><scope>H8D</scope><scope>L7M</scope></search><sort><creationdate>20150313</creationdate><title>Signatures of molecular orbital structure in lateral electron momentum distributions from strong-field ionization</title><author>Petersen, Ingo ; Henkel, Jost ; Lein, Manfred</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c511t-a91e6202df28d84ec7a7138fe677977863171ab45a27ae34c0c9be632cc52d143</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Angular distribution</topic><topic>Angular momentum</topic><topic>Ionization</topic><topic>Lasers</topic><topic>Mathematical analysis</topic><topic>Molecular orbitals</topic><topic>Planes</topic><topic>Signatures</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Petersen, Ingo</creatorcontrib><creatorcontrib>Henkel, Jost</creatorcontrib><creatorcontrib>Lein, Manfred</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Physical review letters</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Petersen, Ingo</au><au>Henkel, Jost</au><au>Lein, Manfred</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Signatures of molecular orbital structure in lateral electron momentum distributions from strong-field ionization</atitle><jtitle>Physical review letters</jtitle><addtitle>Phys Rev Lett</addtitle><date>2015-03-13</date><risdate>2015</risdate><volume>114</volume><issue>10</issue><spage>103004</spage><epage>103004</epage><pages>103004-103004</pages><artnum>103004</artnum><issn>0031-9007</issn><eissn>1079-7114</eissn><abstract>Strong-field ionization of aligned diatomic and polyatomic molecules such as O2, N2, C2H4, and others in circularly polarized laser fields is investigated theoretically. By calculating the emission-angle-resolved lateral width of the momentum distribution perpendicular to the polarization plane, we show that nodal planes in molecular orbitals are directly imprinted on the angular dependence of the width. We demonstrate that orbital symmetries can be distinguished with the information obtained by observing the lateral width in addition to the angular distributions.</abstract><cop>United States</cop><pmid>25815929</pmid><doi>10.1103/physrevlett.114.103004</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 0031-9007 |
| ispartof | Physical review letters, 2015-03, Vol.114 (10), p.103004-103004, Article 103004 |
| issn | 0031-9007 1079-7114 |
| language | eng |
| recordid | cdi_proquest_miscellaneous_1786221529 |
| source | American Physical Society Journals |
| subjects | Angular distribution Angular momentum Ionization Lasers Mathematical analysis Molecular orbitals Planes Signatures |
| title | Signatures of molecular orbital structure in lateral electron momentum distributions from strong-field ionization |
| url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-08T15%3A22%3A00IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Signatures%20of%20molecular%20orbital%20structure%20in%20lateral%20electron%20momentum%20distributions%20from%20strong-field%20ionization&rft.jtitle=Physical%20review%20letters&rft.au=Petersen,%20Ingo&rft.date=2015-03-13&rft.volume=114&rft.issue=10&rft.spage=103004&rft.epage=103004&rft.pages=103004-103004&rft.artnum=103004&rft.issn=0031-9007&rft.eissn=1079-7114&rft_id=info:doi/10.1103/physrevlett.114.103004&rft_dat=%3Cproquest_cross%3E1667965926%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1667965926&rft_id=info:pmid/25815929&rfr_iscdi=true |