Visible-light, photoredox catalyzed, oxidative hydroxylation of arylboronic acids using a metal-organic framework containing tetrakis(carboxyphenyl)porphyrin groups

Visible-light, photoredox catalyzed, oxidative hydroxylation of arylboronic acids using a metal-organic framework containing tetrakis(carboxyphenyl)porphyrin groups

A Zr-based metal-organic framework with tetrakis(carboxyphenyl)porphyrin groups (Zr-MOF-TCPP: MOF-525) has been utilized as a photoredox catalyst to promote oxidative hydroxylation of arylboronic acids under green LED light irradiation. Zr-MOF-TCPP displays a superior catalytic activity for this pro...

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Veröffentlicht in:Chemical communications (Cambridge, England) England), 2015-01, Vol.51 (89), p.16103-16106
Hauptverfasser: Toyao, Takashi, Ueno, Nana, Miyahara, Kenta, Matsui, Yasunori, Kim, Tae-Ho, Horiuchi, Yu, Ikeda, Hiroshi, Matsuoka, Masaya
Format: Artikel
Sprache:eng
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Catalysts
Catalytic activity
Displays
Hydroxylation
Light irradiation
Light-emitting diodes
Metal-organic frameworks
Metalorganic compounds
Zirconium
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container_end_page 16106
container_issue 89
container_start_page 16103
container_title Chemical communications (Cambridge, England)
container_volume 51
creator Toyao, Takashi
Ueno, Nana
Miyahara, Kenta
Matsui, Yasunori
Kim, Tae-Ho
Horiuchi, Yu
Ikeda, Hiroshi
Matsuoka, Masaya
description A Zr-based metal-organic framework with tetrakis(carboxyphenyl)porphyrin groups (Zr-MOF-TCPP: MOF-525) has been utilized as a photoredox catalyst to promote oxidative hydroxylation of arylboronic acids under green LED light irradiation. Zr-MOF-TCPP displays a superior catalytic activity for this process over the corresponding homogeneous catalyst (H4TCPP).
doi_str_mv 10.1039/c5cc06163f
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source Royal Society Of Chemistry Journals; Alma/SFX Local Collection
subjects Catalysts
Catalytic activity
Displays
Hydroxylation
Light irradiation
Light-emitting diodes
Metal-organic frameworks
Metalorganic compounds
Zirconium
title Visible-light, photoredox catalyzed, oxidative hydroxylation of arylboronic acids using a metal-organic framework containing tetrakis(carboxyphenyl)porphyrin groups
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