Lasing action in strongly coupled plasmonic nanocavity arrays

Periodic dielectric structures are typically integrated with a planar waveguide to create photonic band-edge modes for feedback in one-dimensional distributed feedback lasers and two-dimensional photonic-crystal lasers 1 , 2 , 3 , 4 . Although photonic band-edge lasers are widely used in optics and...

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Veröffentlicht in:Nat Nano 2013-07, Vol.8 (7), p.506-511
Hauptverfasser: Zhou, Wei, Dridi, Montacer, Suh, Jae Yong, Kim, Chul Hoon, Co, Dick T., Wasielewski, Michael R., Schatz, George C., Odom, Teri W.
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Sprache:eng
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Zusammenfassung:Periodic dielectric structures are typically integrated with a planar waveguide to create photonic band-edge modes for feedback in one-dimensional distributed feedback lasers and two-dimensional photonic-crystal lasers 1 , 2 , 3 , 4 . Although photonic band-edge lasers are widely used in optics and biological applications, drawbacks include low modulation speeds and diffraction-limited mode confinement 5 , 6 . In contrast, plasmonic nanolasers can support ultrafast dynamics and ultrasmall mode volumes 7 , 8 , 9 . However, because of the large momentum mismatch between their nanolocalized lasing fields and free-space light, they suffer from large radiative losses and lack beam directionality. Here, we report lasing action from band-edge lattice plasmons in arrays of plasmonic nanocavities in a homogeneous dielectric environment. We find that optically pumped, two-dimensional arrays of plasmonic Au or Ag nanoparticles surrounded by an organic gain medium show directional beam emission (divergence angle
ISSN:1748-3387
1748-3395
DOI:10.1038/nnano.2013.99