A Preliminary Study of Oceanic Bomb Radiocarbon Inventory in the North Pacific during the Last Two Decades

Radiocarbon and total carbonate data were obtained near the 1973 GEOSECS stations in the North Pacific along 30°N and along 175°E between 1993 and 1994. In these stations, we estimated radiocarbon originating from atomic bomb tests using tritium, trichlorofluoromethane and silicate contents. The average penetration depth of bomb radiocarbon during the two decades has deepened from 900 m to 1300 m. Bomb radiocarbon inventories above the average value for the whole North Pacific were found widely in the western subtropical region around 30°N both in the 1970s and 1990s, and its area in the 1990s was broader than that in the 1970s. In most of the North Pacific, while the bomb radiocarbon has decreased above 25.4σ^sub [theta]^, the bomb radiocarbon flux below 25.4σ^sub [theta]^ was over 1 × 10^sup 12^ atom m^sup -2^yr^sup -1^ in the subtropical region around 30°N. In the tropical area south of 20°N, the bomb radiocarbon inventory below 25.4σ^sub [theta]^ increased from zero to over 10 × 10^sup 12^ atom m^sup -2^ during the last three decades. These distributions suggest that the bomb radiocarbon removed from the surface is currently accumulated with bomb ^sup 14^C flux of over 1 × 10^sup 12^ atom m^sup -2^yr^sup -1^ below 25.4σ^sub [theta]^ in the subtropical region, mainly by advection from the higher latitude, and that part of the accumulated bomb ^sup 14^C gradually spread southward with about 30 years.[PUBLICATION ABSTRACT]