Chemical Management for Colorful, Efficient, and Stable Inorganic–Organic Hybrid Nanostructured Solar Cells
Chemically tuned inorganic–organic hybrid materials, based on CH3NH3(MA)Pb(I1–x Br x )3 perovskites, have been studied using UV–vis absorption and X-ray diffraction patterns and applied to nanostructured solar cells. The band gap engineering brought about by the chemical management of MAPb(I1–x Br...
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Veröffentlicht in: | Nano letters 2013-04, Vol.13 (4), p.1764-1769 |
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Sprache: | eng |
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Zusammenfassung: | Chemically tuned inorganic–organic hybrid materials, based on CH3NH3(MA)Pb(I1–x Br x )3 perovskites, have been studied using UV–vis absorption and X-ray diffraction patterns and applied to nanostructured solar cells. The band gap engineering brought about by the chemical management of MAPb(I1–x Br x )3 perovskites can be controllably tuned to cover almost the entire visible spectrum, enabling the realization of colorful solar cells. We demonstrate highly efficient solar cells exhibiting 12.3% in a power conversion efficiency of under standard AM 1.5, for the most efficient device, as a result of tunable composition for the light harvester in conjunction with a mesoporous TiO2 film and a hole conducting polymer. We believe that the works highlighted in this paper represent one step toward the realization of low-cost, high-efficiency, and long-term stability with colorful solar cells. |
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ISSN: | 1530-6984 1530-6992 |
DOI: | 10.1021/nl400349b |