Theory of inelastic neutron scattering in a field-induced spin-nematic state

We develop a theory of spin excitations in a field-induced spin-nematic state, and use it to show how a spin-nematic order can be indentified using inelastic neutron scattering. We concentrate on two-dimensional frustrated ferromagnets, for which a two-sublattice, bond-centered spin-nematic state is...

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Veröffentlicht in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2015-05, Vol.91 (17), Article 174402
Hauptverfasser: Smerald, Andrew, Ueda, Hiroaki T., Shannon, Nic
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Sprache:eng
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Zusammenfassung:We develop a theory of spin excitations in a field-induced spin-nematic state, and use it to show how a spin-nematic order can be indentified using inelastic neutron scattering. We concentrate on two-dimensional frustrated ferromagnets, for which a two-sublattice, bond-centered spin-nematic state is predicted to exist over a wide range of parameters. First, to clarify the nature of spin-excitations, we introduce a soluble spin-1 model, and use this to derive a continuum field theory, applicable to any two-sublattice spin-nematic state. We then parameterize this field theory, using diagrammatic calculations for a realistic microscopic model of a spin-1/2 frustrated ferromagnet, and show how it can be used to make predictions for inelastic neutron scattering. As an example, we show quantitative predictions for inelastic scattering of neutrons from BaCdVO(PO sub(4)) sub(2), a promising candidate to realize a spin-nematic state at an achievable h ~ 4 T. We show that in this material it is realistic to expect a ghostly Goldstone mode, signalling spin-nematic order, to be visible in experiment.
ISSN:1098-0121
1550-235X
DOI:10.1103/PhysRevB.91.174402