Oxygen-content-dependent electronic structures of electron-doped cuprates
We performed systematic angle-resolved photoemission studies on as-grown and oxygen-reduced electron-doped cuprates Pr sub(0.85)LaCe sub(0.15)CuO sub(4), Nd sub(1.85)Ce sub(0.15)CuO sub(4), and Sm sub(1.85)Ce sub(0.15)CuO sub(4), in order to investigate the oxygen-reduction process. All of the as-gr...
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Veröffentlicht in: | Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2012-10, Vol.86 (14) |
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Hauptverfasser: | , , , , , , , , , , , , , |
Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | We performed systematic angle-resolved photoemission studies on as-grown and oxygen-reduced electron-doped cuprates Pr sub(0.85)LaCe sub(0.15)CuO sub(4), Nd sub(1.85)Ce sub(0.15)CuO sub(4), and Sm sub(1.85)Ce sub(0.15)CuO sub(4), in order to investigate the oxygen-reduction process. All of the as-grown systems we have studied show metallic edges in the antinodal region, while near E sub(F) nodal spectra are suppressed, resulting in partial gap opening. In addition, spectra from as-grown systems show weak and broad low-energy quasiparticle peaks (QPPs). Upon proper reduction, sharp QPPs emerge but they are strongly suppressed again in the over-reduced state. This QPP behavior deviates from the magnetism and doping-evolution origin of QPP suppression, and implies that scattering due to disorder and impurity is a more probable cause for the broken coherence of the quasiparticle state. Our results are also consistent with the recently proposed Cu-deficiency scenario. |
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ISSN: | 1098-0121 1550-235X |