Inelastic Neutron Scattering Investigation in Glassy SiSe2: Complex Dynamics at the Atomic Scale

A detailed investigation of the THz dynamics in glassy SiSe2 by means of neutron inelastic scattering is presented. To carefully map the translational dynamics and the region of the boson peak, we carried out two different experiments with sharp and broad resolutions coupled with a narrow and a wide...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:The journal of physical chemistry letters 2013-04, Vol.4 (7), p.1143-1147
Hauptverfasser: Zanatta, Marco, Fontana, A, Orecchini, A, Petrillo, C, Sacchetti, F
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
Beschreibung
Zusammenfassung:A detailed investigation of the THz dynamics in glassy SiSe2 by means of neutron inelastic scattering is presented. To carefully map the translational dynamics and the region of the boson peak, we carried out two different experiments with sharp and broad resolutions coupled with a narrow and a wide kinematic range, respectively. Data show a complex pattern of excitations made up of three components. The most intense one is the prolongation of the longitudinal acoustic mode while two other modes appear in the boson peak region below 3 meV. We propose an interaction model that allows for a consistent identification of the nature of these modes.
ISSN:1948-7185
1948-7185
DOI:10.1021/jz400232c