A Water-Stable Porphyrin-Based Metal-Organic Framework Active for Visible-Light Photocatalysis
Light‐harvesting MOFs: A new porous porphyrinic metal–organic framework (MOF; see picture) was obtained by hydrothermal synthesis. The chemical and thermal stability of the material allows a postsynthetic insertion of zinc in the center of the porphyrin. The visible‐light photocatalytic activity of...
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| Veröffentlicht in: | Angewandte Chemie International Edition 2012-07, Vol.51 (30), p.7440-7444 |
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| container_title | Angewandte Chemie International Edition |
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| creator | Fateeva, Alexandra Chater, Philip A. Ireland, Christopher P. Tahir, Asif A. Khimyak, Yaroslav Z. Wiper, Paul V. Darwent, James R. Rosseinsky, Matthew J. |
| description | Light‐harvesting MOFs: A new porous porphyrinic metal–organic framework (MOF; see picture) was obtained by hydrothermal synthesis. The chemical and thermal stability of the material allows a postsynthetic insertion of zinc in the center of the porphyrin. The visible‐light photocatalytic activity of this porphyrin‐based material is shown for the sacrificial hydrogen evolution from water. |
| doi_str_mv | 10.1002/anie.201202471 |
| format | Article |
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| source | Wiley Online Library Journals Frontfile Complete |
| subjects | heterogeneous catalysis Hydrogen evolution hydrogen production Insertion Metal-organic frameworks Photocatalysis Pictures porphyrinoids Porphyrins Synthesis Thermal stability Zinc |
| title | A Water-Stable Porphyrin-Based Metal-Organic Framework Active for Visible-Light Photocatalysis |
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