Carbon for the oxygen reduction reaction: a defect mechanism

We demonstrate a new defect mechanism of carbons for the oxygen reduction reaction (ORR). It is predicted by the first principles calculations that a type of 585 defect on graphene (G585) is more effective than N-doping for the ORR, and our experimental investigations show strong support to this the...

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Veröffentlicht in:Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2015-01, Vol.3 (22), p.11736-11739
Hauptverfasser: Zhao, Huanyu, Sun, Chenghua, Jin, Zhao, Wang, Da-Wei, Yan, Xuecheng, Chen, Zhigang, Zhu, Guangshan, Yao, Xiangdong
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Sprache:eng
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Zusammenfassung:We demonstrate a new defect mechanism of carbons for the oxygen reduction reaction (ORR). It is predicted by the first principles calculations that a type of 585 defect on graphene (G585) is more effective than N-doping for the ORR, and our experimental investigations show strong support to this theoretical prediction.
ISSN:2050-7488
2050-7496
DOI:10.1039/c5ta02229k