Spin and charge dynamics of a quasi-one-dimensional antiferromagnetic metal

We use quantum Monte Carlo simulations to study a finite-temperature dimensional-crossover-driven evolution of spin and charge dynamics in an anisotropic two-dimensional system of weakly coupled Hubbard chains with a half-filled band. The low-temperature behavior of the charge gap indicates a crosso...

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Veröffentlicht in:Physical review. B, Condensed matter and materials physics Condensed matter and materials physics, 2015-01, Vol.91 (4), Article 045137
Hauptverfasser: Raczkowski, Marcin, Assaad, Fakher F., Pollet, Lode
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Sprache:eng
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Zusammenfassung:We use quantum Monte Carlo simulations to study a finite-temperature dimensional-crossover-driven evolution of spin and charge dynamics in an anisotropic two-dimensional system of weakly coupled Hubbard chains with a half-filled band. The low-temperature behavior of the charge gap indicates a crossover between two distinct energy scales: a high-energy one-dimensional (1D) Mott gap due to the umklapp process and a low-energy gap which stems from long-range antiferromagnetic (AF) spin fluctuations. Away from the 1D regime and at temperature scales above the charge gap, the emergence of a zero-frequency Drude-like feature in the interchain optical conductivity [sigma] sub([perpendicular])( omega ) implies the onset of a higher-dimensional metal. In this metallic phase, enhanced quasiparticle scattering off finite-range AF spin fluctuations results in incoherent single-particle dynamics. The coupling between spin and charge fluctuations is also seen in the spin dynamical structure factor S(q, omega ) displaying damped spin excitations (paramagnons) close to the AF wave vector q = ([pi], [pi]) and particle-hole continua near 1D momentum transfers spanning quasiparticles at the Fermi surface. We relate our results to the charge deconfinement in quasi-1D organic Bechgaard-Fabre salts.
ISSN:1098-0121
1550-235X
DOI:10.1103/PhysRevB.91.045137