Spatio-temporal variation of biogenic volatile organic compounds emissions in China

Aiming to reduce the large uncertainties of biogenic volatile organic compounds (BVOCs) emissions estimation, the emission inventory of BVOCs in China at a high spatial and temporal resolution of 36 km × 36 km and 1 h was established using MEGANv2.1 with MM5 providing high-resolution meteorological...

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Veröffentlicht in:Environmental pollution (1987) 2013-11, Vol.182, p.157-168
Hauptverfasser: Li, L.Y., Chen, Y., Xie, S.D.
Format: Artikel
Sprache:eng
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Zusammenfassung:Aiming to reduce the large uncertainties of biogenic volatile organic compounds (BVOCs) emissions estimation, the emission inventory of BVOCs in China at a high spatial and temporal resolution of 36 km × 36 km and 1 h was established using MEGANv2.1 with MM5 providing high-resolution meteorological data, based on the most detailed and latest vegetation investigations. BVOC emissions from 82 plant functional types in China were computed firstly. More local species-specific emission rates were developed combining statistical analysis and category classification, and the leaf biomass was estimated based on vegetation volume and production with biomass-apportion models. The total annual BVOC emissions in 2003 were 42.5 Tg, including isoprene 23.4 Tg, monoterpene 5.6 Tg, sesquiterpene 1.0 Tg, and other VOCs (OVOCs) 12.5 Tg. Subtropical and tropical evergreen and deciduous broadleaf shrubs, Quercus, and bamboo contributed more than 45% to the total BVOC emissions. The highest biogenic emissions were found over northeastern, southeastern, and southwestern China. Strong seasonal pattern was observed with the highest BVOC emissions in July and the lowest in January and December, with daily emission peaked at approximately 13:00 or 14:00 local time. •An emission inventory of BVOCs in China at a high spatial and temporal resolution of 36 km and 1 h is established.•High-resolution meteorological data simulated by MM5 is used.•We update the land cover data used in MEGAN based on the most detailed and latest vegetation investigations.•A new vegetation classification with 82 plant functional types is developed in MEGAN.•The leaf biomass is estimated based on vegetation volume and production with biomass-apportion models. An emission inventory of BVOCs in China was established based on the most detailed and latest vegetation investigations, and high-resolution meteorological data.
ISSN:0269-7491
1873-6424
DOI:10.1016/j.envpol.2013.06.042