A secular technetium–molybdenum generator
A compact secular molybdenium generator is subject of this paper. This generator represents a nuclear system that comprises a hydrogen-isotopes fusor, moderator, reflector and shield. Deuterium fusion reactions in a tritiated or deuterated target provide the neutron source. A moderation fluid slowdo...
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Veröffentlicht in: | Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment Accelerators, spectrometers, detectors and associated equipment, 2015-05, Vol.782, p.40-46 |
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Hauptverfasser: | , |
Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | A compact secular molybdenium generator is subject of this paper. This generator represents a nuclear system that comprises a hydrogen-isotopes fusor, moderator, reflector and shield. Deuterium fusion reactions in a tritiated or deuterated target provide the neutron source. A moderation fluid slowdown the neutron energy which increases 98Mo(n,γ)99Mo capture reaction rates. Neutron reflection minimizes the neutron escape and the radiation shield encloses the device. The neutron yield calculation along with electromagnetic and nuclear simulations were addressed. Results revealed the accelerator equipotential surfaces ranging from −30 to 150kV, the ion trajectories and the energy beam profile define a deuteron current of 1A with energy of 180keV at the target, the spatial distribution of the neutron flux, and the 99Mo and 99mTc activities in function of transmuter operation time. The kinetics of the 99mTc correlated to its precursor activity demonstrates a secular equilibrium providing 2 Ci in a operational time of 150h. As conclusion, the investigated nuclear and electromagnetic features have demonstrated that such generator shall have a notable potential for feeding the 99mTc clinical application. |
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ISSN: | 0168-9002 1872-9576 |
DOI: | 10.1016/j.nima.2015.01.095 |