Kinetic analysis of constructed systems for the recovery of contaminated areas by acid mine drainage
Introduction Flowing of the acid mine drainage may contaminate the adjacent water bodies causing substantial changes in the aquatic ecosystem. This aspect is the most relevant problem in the southern of Santa Catarina once the contaminated areas are inserted in the watershed of the Araranguá, Urussa...
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| Veröffentlicht in: | Environmental science and pollution research international 2012-07, Vol.19 (6), p.2107-2114 |
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| creator | Mendes, Erlon Barros, Erilson Zocche, Jairo José Alexandre, Nadja Zim Galatto, Sérgio Luciano Back, Marcos Pereira, Jader Lima Frassetto, Jonathan Angioletto, Elidio |
| description | Introduction
Flowing of the acid mine drainage may contaminate the adjacent water bodies causing substantial changes in the aquatic ecosystem. This aspect is the most relevant problem in the southern of Santa Catarina once the contaminated areas are inserted in the watershed of the Araranguá, Urussanga, and Tubarão rivers, increasing the need for recovery studies. These areas are between Criciúma, Içara, Urussanga, Siderópolis, Lauro Müller, Orleans, and Alfredo Wagner towns where a conservation unit exist called the Environmental Preservation Area of Baleia Franca. Aiming to compare the kinetics of the ash derived from burning coal and to neutralize acid mine drainage, different neutralizer, limestone, fly, and bottom ash, was mounted on a pilot scale experiment.
Discussion
The transport parameters showed the same order of infiltration and dispersion: fly ash < bottom ash < limestone. The order of measured alkalinity was: limestone < fly ash < bottom ash, with pH values of 9.34, 12.07, and 12.25, respectively. The limestone kinetics of acidic drainage neutralization was first order with reaction rate constant
k
= 0.0963 min
−1
, bottom ash was 3/4 with
k
= 0.0723 mol
1/4
L
−1/4
min
−1
, and the fly ash had higher order kinetics, 4/3, with reaction rate constant
k
= 27.122 L
1/3
mol
−1/3
min
−1
. However, by mathematical modeling, it was found that due to a combination of transport and kinetics, only limestone treatment reached a pH above 6 within 5 years, corresponding to the ideal as planned. |
| doi_str_mv | 10.1007/s11356-011-0710-2 |
| format | Article |
| fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1671608172</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2704079191</sourcerecordid><originalsourceid>FETCH-LOGICAL-c390t-b3077f9941ae94988dea25d3bf057be933e81adc24d98c15796468bd28855f853</originalsourceid><addsrcrecordid>eNqF0c-L1TAQB_Agivtc_QO8SMCLl7ozSdokR1n8hQt7cc8lTaZrl9d2zbRC_3vz9j1FBDGXQOaTmZCvEC8R3iKAvWBEXTcVIFZgESr1SOywQVNZ4_1jsQNvTIXamDPxjPkOQIFX9qk4U2VZB3Yn0pdhomWIMkxhv_HAcu5lnCde8hoXSpI3Xmhk2c9ZLt9IZorzD8rbyS1hHKZwgCFTYNltMsQhyXJKMuVQirf0XDzpw57pxWk_Fzcf3n-9_FRdXX_8fPnuqoraw1J1GqztvTcYyBvvXKKg6qS7HmrbkdeaHIYUlUneRaytb0zjuqScq-ve1fpcvDn2vc_z95V4aceBI-33YaJ55RYbiw04tOr_FJQDjeBMoa__onfzmst3PShtDRj0ReFRxTwzZ-rb-zyMIW8FtYe02mNabUmrPaTVHh7x6tR57UZKv2_8iqcAdQRcStMt5T9H_6vrT91hnmE</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1023740419</pqid></control><display><type>article</type><title>Kinetic analysis of constructed systems for the recovery of contaminated areas by acid mine drainage</title><source>MEDLINE</source><source>SpringerLink Journals - AutoHoldings</source><creator>Mendes, Erlon ; Barros, Erilson ; Zocche, Jairo José ; Alexandre, Nadja Zim ; Galatto, Sérgio Luciano ; Back, Marcos ; Pereira, Jader Lima ; Frassetto, Jonathan ; Angioletto, Elidio</creator><creatorcontrib>Mendes, Erlon ; Barros, Erilson ; Zocche, Jairo José ; Alexandre, Nadja Zim ; Galatto, Sérgio Luciano ; Back, Marcos ; Pereira, Jader Lima ; Frassetto, Jonathan ; Angioletto, Elidio</creatorcontrib><description>Introduction
Flowing of the acid mine drainage may contaminate the adjacent water bodies causing substantial changes in the aquatic ecosystem. This aspect is the most relevant problem in the southern of Santa Catarina once the contaminated areas are inserted in the watershed of the Araranguá, Urussanga, and Tubarão rivers, increasing the need for recovery studies. These areas are between Criciúma, Içara, Urussanga, Siderópolis, Lauro Müller, Orleans, and Alfredo Wagner towns where a conservation unit exist called the Environmental Preservation Area of Baleia Franca. Aiming to compare the kinetics of the ash derived from burning coal and to neutralize acid mine drainage, different neutralizer, limestone, fly, and bottom ash, was mounted on a pilot scale experiment.
Discussion
The transport parameters showed the same order of infiltration and dispersion: fly ash < bottom ash < limestone. The order of measured alkalinity was: limestone < fly ash < bottom ash, with pH values of 9.34, 12.07, and 12.25, respectively. The limestone kinetics of acidic drainage neutralization was first order with reaction rate constant
k
= 0.0963 min
−1
, bottom ash was 3/4 with
k
= 0.0723 mol
1/4
L
−1/4
min
−1
, and the fly ash had higher order kinetics, 4/3, with reaction rate constant
k
= 27.122 L
1/3
mol
−1/3
min
−1
. However, by mathematical modeling, it was found that due to a combination of transport and kinetics, only limestone treatment reached a pH above 6 within 5 years, corresponding to the ideal as planned.</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-011-0710-2</identifier><identifier>PMID: 22227807</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer-Verlag</publisher><subject>Acid mine drainage ; Alkalinity ; Aquatic ecosystems ; Aquatic Pollution ; Ashes ; Atmospheric Protection/Air Quality Control/Air Pollution ; Brazil ; By products ; Coal ; Coal Ash - metabolism ; Coal Mining ; Contamination ; Earth and Environmental Science ; Ecosystem recovery ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental impact ; Environmental Restoration and Remediation - methods ; Experiments ; Fly ash ; Hazardous materials ; Hydrogen-Ion Concentration ; Kinetics ; Landfill ; Limestone ; Mathematical models ; Mine drainage ; Neutralization ; Oxidation ; Pilot Projects ; Rain ; Reaction kinetics ; Research Article ; Studies ; Waste Water Technology ; Water Management ; Water Pollution Control</subject><ispartof>Environmental science and pollution research international, 2012-07, Vol.19 (6), p.2107-2114</ispartof><rights>Springer-Verlag 2012</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c390t-b3077f9941ae94988dea25d3bf057be933e81adc24d98c15796468bd28855f853</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11356-011-0710-2$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s11356-011-0710-2$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,780,784,27923,27924,41487,42556,51318</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/22227807$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Mendes, Erlon</creatorcontrib><creatorcontrib>Barros, Erilson</creatorcontrib><creatorcontrib>Zocche, Jairo José</creatorcontrib><creatorcontrib>Alexandre, Nadja Zim</creatorcontrib><creatorcontrib>Galatto, Sérgio Luciano</creatorcontrib><creatorcontrib>Back, Marcos</creatorcontrib><creatorcontrib>Pereira, Jader Lima</creatorcontrib><creatorcontrib>Frassetto, Jonathan</creatorcontrib><creatorcontrib>Angioletto, Elidio</creatorcontrib><title>Kinetic analysis of constructed systems for the recovery of contaminated areas by acid mine drainage</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>Introduction
Flowing of the acid mine drainage may contaminate the adjacent water bodies causing substantial changes in the aquatic ecosystem. This aspect is the most relevant problem in the southern of Santa Catarina once the contaminated areas are inserted in the watershed of the Araranguá, Urussanga, and Tubarão rivers, increasing the need for recovery studies. These areas are between Criciúma, Içara, Urussanga, Siderópolis, Lauro Müller, Orleans, and Alfredo Wagner towns where a conservation unit exist called the Environmental Preservation Area of Baleia Franca. Aiming to compare the kinetics of the ash derived from burning coal and to neutralize acid mine drainage, different neutralizer, limestone, fly, and bottom ash, was mounted on a pilot scale experiment.
Discussion
The transport parameters showed the same order of infiltration and dispersion: fly ash < bottom ash < limestone. The order of measured alkalinity was: limestone < fly ash < bottom ash, with pH values of 9.34, 12.07, and 12.25, respectively. The limestone kinetics of acidic drainage neutralization was first order with reaction rate constant
k
= 0.0963 min
−1
, bottom ash was 3/4 with
k
= 0.0723 mol
1/4
L
−1/4
min
−1
, and the fly ash had higher order kinetics, 4/3, with reaction rate constant
k
= 27.122 L
1/3
mol
−1/3
min
−1
. However, by mathematical modeling, it was found that due to a combination of transport and kinetics, only limestone treatment reached a pH above 6 within 5 years, corresponding to the ideal as planned.</description><subject>Acid mine drainage</subject><subject>Alkalinity</subject><subject>Aquatic ecosystems</subject><subject>Aquatic Pollution</subject><subject>Ashes</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Brazil</subject><subject>By products</subject><subject>Coal</subject><subject>Coal Ash - metabolism</subject><subject>Coal Mining</subject><subject>Contamination</subject><subject>Earth and Environmental Science</subject><subject>Ecosystem recovery</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental impact</subject><subject>Environmental Restoration and Remediation - methods</subject><subject>Experiments</subject><subject>Fly ash</subject><subject>Hazardous materials</subject><subject>Hydrogen-Ion Concentration</subject><subject>Kinetics</subject><subject>Landfill</subject><subject>Limestone</subject><subject>Mathematical models</subject><subject>Mine drainage</subject><subject>Neutralization</subject><subject>Oxidation</subject><subject>Pilot Projects</subject><subject>Rain</subject><subject>Reaction kinetics</subject><subject>Research Article</subject><subject>Studies</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollution 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Erilson</creator><creator>Zocche, Jairo José</creator><creator>Alexandre, Nadja Zim</creator><creator>Galatto, Sérgio Luciano</creator><creator>Back, Marcos</creator><creator>Pereira, Jader Lima</creator><creator>Frassetto, Jonathan</creator><creator>Angioletto, Elidio</creator><general>Springer-Verlag</general><general>Springer Nature 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Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2012-07-01</date><risdate>2012</risdate><volume>19</volume><issue>6</issue><spage>2107</spage><epage>2114</epage><pages>2107-2114</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>Introduction
Flowing of the acid mine drainage may contaminate the adjacent water bodies causing substantial changes in the aquatic ecosystem. This aspect is the most relevant problem in the southern of Santa Catarina once the contaminated areas are inserted in the watershed of the Araranguá, Urussanga, and Tubarão rivers, increasing the need for recovery studies. These areas are between Criciúma, Içara, Urussanga, Siderópolis, Lauro Müller, Orleans, and Alfredo Wagner towns where a conservation unit exist called the Environmental Preservation Area of Baleia Franca. Aiming to compare the kinetics of the ash derived from burning coal and to neutralize acid mine drainage, different neutralizer, limestone, fly, and bottom ash, was mounted on a pilot scale experiment.
Discussion
The transport parameters showed the same order of infiltration and dispersion: fly ash < bottom ash < limestone. The order of measured alkalinity was: limestone < fly ash < bottom ash, with pH values of 9.34, 12.07, and 12.25, respectively. The limestone kinetics of acidic drainage neutralization was first order with reaction rate constant
k
= 0.0963 min
−1
, bottom ash was 3/4 with
k
= 0.0723 mol
1/4
L
−1/4
min
−1
, and the fly ash had higher order kinetics, 4/3, with reaction rate constant
k
= 27.122 L
1/3
mol
−1/3
min
−1
. However, by mathematical modeling, it was found that due to a combination of transport and kinetics, only limestone treatment reached a pH above 6 within 5 years, corresponding to the ideal as planned.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer-Verlag</pub><pmid>22227807</pmid><doi>10.1007/s11356-011-0710-2</doi><tpages>8</tpages></addata></record> |
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| ispartof | Environmental science and pollution research international, 2012-07, Vol.19 (6), p.2107-2114 |
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| source | MEDLINE; SpringerLink Journals - AutoHoldings |
| subjects | Acid mine drainage Alkalinity Aquatic ecosystems Aquatic Pollution Ashes Atmospheric Protection/Air Quality Control/Air Pollution Brazil By products Coal Coal Ash - metabolism Coal Mining Contamination Earth and Environmental Science Ecosystem recovery Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental impact Environmental Restoration and Remediation - methods Experiments Fly ash Hazardous materials Hydrogen-Ion Concentration Kinetics Landfill Limestone Mathematical models Mine drainage Neutralization Oxidation Pilot Projects Rain Reaction kinetics Research Article Studies Waste Water Technology Water Management Water Pollution Control |
| title | Kinetic analysis of constructed systems for the recovery of contaminated areas by acid mine drainage |
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