Methanol from CO2 by Organo-Cocatalysis: CO2 Capture and Hydrogenation in One Process Step

Carbon dioxide chemically bound to alcohol-amines was hydrogenated to methanol under retrieval of these industrially used CO2 capturing reagents. The energetics of the process can be seen as a partial cancellation of the exothermic heat of reaction of the hydrogenation with the endothermic one of th...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Environmental science & technology 2014-12, Vol.48 (24), p.14799-14804
Hauptverfasser: Reller, Christian, Pöge, Matthias, Lißner, Andreas, Mertens, Florian O. R. L
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 14804
container_issue 24
container_start_page 14799
container_title Environmental science & technology
container_volume 48
creator Reller, Christian
Pöge, Matthias
Lißner, Andreas
Mertens, Florian O. R. L
description Carbon dioxide chemically bound to alcohol-amines was hydrogenated to methanol under retrieval of these industrially used CO2 capturing reagents. The energetics of the process can be seen as a partial cancellation of the exothermic heat of reaction of the hydrogenation with the endothermic one of the CO2 release from the capturing reagent. The process provides a means to significantly improve the energy efficiency of CO2 to methanol conversions.
doi_str_mv 10.1021/es503914d
format Article
fullrecord <record><control><sourceid>proquest_pubme</sourceid><recordid>TN_cdi_proquest_miscellaneous_1637568466</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1637568466</sourcerecordid><originalsourceid>FETCH-LOGICAL-a337t-5cc26d531d52c83d89fb235714968193e475896caf8ce117c691291392199e2d3</originalsourceid><addsrcrecordid>eNpF0cFKxDAQBuAgiq6rB19AchG8VDOZJk28SVFXUFZQQbyUbJqulW6yJu1h395VVz0NzHwMzPyEHAE7A8bh3CXBUENeb5ERCM4yoQRskxFjgJlG-bJH9lN6Z4xxZGqX7HGBWhY5jsjrvevfjA8dbWJY0HLK6WxFp3G-7mVlsKY33Sq16eJ7VJplP0RHja_pZFXHMHfe9G3wtPV06h19iMG6lOhj75YHZKcxXXKHmzomz9dXT-Uku5ve3JaXd5lBLPpMWMtlLRBqwa3CWulmxlEUkGupQKPLC6G0tKZR1gEUVmrgGlBz0NrxGsfk9GfvMoaPwaW-WrTJuq4z3oUhVSCxEFLlUq7p8YYOs4Wrq2VsFyauqt9_rMHJBphkTddE422b_p1mSmLO_p2xqXoPQ_TrCytg1Vce1V8e-AmwVXcl</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1637568466</pqid></control><display><type>article</type><title>Methanol from CO2 by Organo-Cocatalysis: CO2 Capture and Hydrogenation in One Process Step</title><source>MEDLINE</source><source>ACS Publications</source><creator>Reller, Christian ; Pöge, Matthias ; Lißner, Andreas ; Mertens, Florian O. R. L</creator><creatorcontrib>Reller, Christian ; Pöge, Matthias ; Lißner, Andreas ; Mertens, Florian O. R. L</creatorcontrib><description>Carbon dioxide chemically bound to alcohol-amines was hydrogenated to methanol under retrieval of these industrially used CO2 capturing reagents. The energetics of the process can be seen as a partial cancellation of the exothermic heat of reaction of the hydrogenation with the endothermic one of the CO2 release from the capturing reagent. The process provides a means to significantly improve the energy efficiency of CO2 to methanol conversions.</description><identifier>ISSN: 0013-936X</identifier><identifier>EISSN: 1520-5851</identifier><identifier>DOI: 10.1021/es503914d</identifier><identifier>PMID: 25396743</identifier><identifier>CODEN: ESTHAG</identifier><language>eng</language><publisher>Washington, DC: American Chemical Society</publisher><subject>Carbon Dioxide - chemistry ; Catalysis ; Catalytic reactions ; Chemistry ; Ethanolamines - chemistry ; Exact sciences and technology ; General and physical chemistry ; Hot Temperature ; Hydrogenation ; Methanol - chemistry ; Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><ispartof>Environmental science &amp; technology, 2014-12, Vol.48 (24), p.14799-14804</ispartof><rights>2015 INIST-CNRS</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://pubs.acs.org/doi/pdf/10.1021/es503914d$$EPDF$$P50$$Gacs$$H</linktopdf><linktohtml>$$Uhttps://pubs.acs.org/doi/10.1021/es503914d$$EHTML$$P50$$Gacs$$H</linktohtml><link.rule.ids>314,780,784,27076,27924,27925,56738,56788</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&amp;idt=29086340$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/25396743$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Reller, Christian</creatorcontrib><creatorcontrib>Pöge, Matthias</creatorcontrib><creatorcontrib>Lißner, Andreas</creatorcontrib><creatorcontrib>Mertens, Florian O. R. L</creatorcontrib><title>Methanol from CO2 by Organo-Cocatalysis: CO2 Capture and Hydrogenation in One Process Step</title><title>Environmental science &amp; technology</title><addtitle>Environ. Sci. Technol</addtitle><description>Carbon dioxide chemically bound to alcohol-amines was hydrogenated to methanol under retrieval of these industrially used CO2 capturing reagents. The energetics of the process can be seen as a partial cancellation of the exothermic heat of reaction of the hydrogenation with the endothermic one of the CO2 release from the capturing reagent. The process provides a means to significantly improve the energy efficiency of CO2 to methanol conversions.</description><subject>Carbon Dioxide - chemistry</subject><subject>Catalysis</subject><subject>Catalytic reactions</subject><subject>Chemistry</subject><subject>Ethanolamines - chemistry</subject><subject>Exact sciences and technology</subject><subject>General and physical chemistry</subject><subject>Hot Temperature</subject><subject>Hydrogenation</subject><subject>Methanol - chemistry</subject><subject>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</subject><issn>0013-936X</issn><issn>1520-5851</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2014</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNpF0cFKxDAQBuAgiq6rB19AchG8VDOZJk28SVFXUFZQQbyUbJqulW6yJu1h395VVz0NzHwMzPyEHAE7A8bh3CXBUENeb5ERCM4yoQRskxFjgJlG-bJH9lN6Z4xxZGqX7HGBWhY5jsjrvevfjA8dbWJY0HLK6WxFp3G-7mVlsKY33Sq16eJ7VJplP0RHja_pZFXHMHfe9G3wtPV06h19iMG6lOhj75YHZKcxXXKHmzomz9dXT-Uku5ve3JaXd5lBLPpMWMtlLRBqwa3CWulmxlEUkGupQKPLC6G0tKZR1gEUVmrgGlBz0NrxGsfk9GfvMoaPwaW-WrTJuq4z3oUhVSCxEFLlUq7p8YYOs4Wrq2VsFyauqt9_rMHJBphkTddE422b_p1mSmLO_p2xqXoPQ_TrCytg1Vce1V8e-AmwVXcl</recordid><startdate>20141216</startdate><enddate>20141216</enddate><creator>Reller, Christian</creator><creator>Pöge, Matthias</creator><creator>Lißner, Andreas</creator><creator>Mertens, Florian O. R. L</creator><general>American Chemical Society</general><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>7X8</scope></search><sort><creationdate>20141216</creationdate><title>Methanol from CO2 by Organo-Cocatalysis: CO2 Capture and Hydrogenation in One Process Step</title><author>Reller, Christian ; Pöge, Matthias ; Lißner, Andreas ; Mertens, Florian O. R. L</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-a337t-5cc26d531d52c83d89fb235714968193e475896caf8ce117c691291392199e2d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2014</creationdate><topic>Carbon Dioxide - chemistry</topic><topic>Catalysis</topic><topic>Catalytic reactions</topic><topic>Chemistry</topic><topic>Ethanolamines - chemistry</topic><topic>Exact sciences and technology</topic><topic>General and physical chemistry</topic><topic>Hot Temperature</topic><topic>Hydrogenation</topic><topic>Methanol - chemistry</topic><topic>Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Reller, Christian</creatorcontrib><creatorcontrib>Pöge, Matthias</creatorcontrib><creatorcontrib>Lißner, Andreas</creatorcontrib><creatorcontrib>Mertens, Florian O. R. L</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science &amp; technology</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Reller, Christian</au><au>Pöge, Matthias</au><au>Lißner, Andreas</au><au>Mertens, Florian O. R. L</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Methanol from CO2 by Organo-Cocatalysis: CO2 Capture and Hydrogenation in One Process Step</atitle><jtitle>Environmental science &amp; technology</jtitle><addtitle>Environ. Sci. Technol</addtitle><date>2014-12-16</date><risdate>2014</risdate><volume>48</volume><issue>24</issue><spage>14799</spage><epage>14804</epage><pages>14799-14804</pages><issn>0013-936X</issn><eissn>1520-5851</eissn><coden>ESTHAG</coden><abstract>Carbon dioxide chemically bound to alcohol-amines was hydrogenated to methanol under retrieval of these industrially used CO2 capturing reagents. The energetics of the process can be seen as a partial cancellation of the exothermic heat of reaction of the hydrogenation with the endothermic one of the CO2 release from the capturing reagent. The process provides a means to significantly improve the energy efficiency of CO2 to methanol conversions.</abstract><cop>Washington, DC</cop><pub>American Chemical Society</pub><pmid>25396743</pmid><doi>10.1021/es503914d</doi><tpages>6</tpages></addata></record>
fulltext fulltext
identifier ISSN: 0013-936X
ispartof Environmental science & technology, 2014-12, Vol.48 (24), p.14799-14804
issn 0013-936X
1520-5851
language eng
recordid cdi_proquest_miscellaneous_1637568466
source MEDLINE; ACS Publications
subjects Carbon Dioxide - chemistry
Catalysis
Catalytic reactions
Chemistry
Ethanolamines - chemistry
Exact sciences and technology
General and physical chemistry
Hot Temperature
Hydrogenation
Methanol - chemistry
Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry
title Methanol from CO2 by Organo-Cocatalysis: CO2 Capture and Hydrogenation in One Process Step
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-06T12%3A43%3A28IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_pubme&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Methanol%20from%20CO2%20by%20Organo-Cocatalysis:%20CO2%20Capture%20and%20Hydrogenation%20in%20One%20Process%20Step&rft.jtitle=Environmental%20science%20&%20technology&rft.au=Reller,%20Christian&rft.date=2014-12-16&rft.volume=48&rft.issue=24&rft.spage=14799&rft.epage=14804&rft.pages=14799-14804&rft.issn=0013-936X&rft.eissn=1520-5851&rft.coden=ESTHAG&rft_id=info:doi/10.1021/es503914d&rft_dat=%3Cproquest_pubme%3E1637568466%3C/proquest_pubme%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1637568466&rft_id=info:pmid/25396743&rfr_iscdi=true