Graphitic carbon nitride nano-emitters on silicon: a photoelectrochemical heterojunction composed of earth-abundant materials for enhanced evolution of hydrogen

Graphitic carbon nitride is a promising heterogeneous catalyst for light-induced generation of hydrogen. Here, we report the successful formation of nano-scaled carbon nitride structures on silicon, mitigating the known limitations of charge transport within bulky C–N networks. An efficient photoele...

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Veröffentlicht in:Journal of materials chemistry. A, Materials for energy and sustainability Materials for energy and sustainability, 2014-08, Vol.2 (32), p.12697-12702
Hauptverfasser: Lublow, M., Fischer, A., Merschjann, C., Yang, F., Schedel-Niedrig, Th, Veyan, J.-F., Chabal, Y. J.
Format: Artikel
Sprache:eng
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Zusammenfassung:Graphitic carbon nitride is a promising heterogeneous catalyst for light-induced generation of hydrogen. Here, we report the successful formation of nano-scaled carbon nitride structures on silicon, mitigating the known limitations of charge transport within bulky C–N networks. An efficient photoelectrochemical heterojunction is thereby realized, developed from earth-abundant materials only.
ISSN:2050-7488
2050-7496
DOI:10.1039/C4TA01711K