Subnanosecond incubation times for electric-field-induced metallization of a correlated electron oxide

Strong interactions, or correlations, between the d or f electrons in transition-metal oxides lead to various types of metal–insulator transitions that can be triggered by external parameters such as temperature, pressure, doping, magnetic fields and electric fields. Electric-field-induced metalliza...

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Veröffentlicht in:Nature nanotechnology 2014-06, Vol.9 (6), p.453-458
Hauptverfasser: Brockman, Justin S., Gao, Li, Hughes, Brian, Rettner, Charles T., Samant, Mahesh G., Roche, Kevin P., Parkin, Stuart S. P.
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Sprache:eng
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Zusammenfassung:Strong interactions, or correlations, between the d or f electrons in transition-metal oxides lead to various types of metal–insulator transitions that can be triggered by external parameters such as temperature, pressure, doping, magnetic fields and electric fields. Electric-field-induced metallization of such materials from their insulating states could enable a new class of ultrafast electronic switches and latches. However, significant questions remain about the detailed nature of the switching process. Here, we show, in the canonical metal-to-insulator transition system V 2 O 3 , that ultrafast voltage pulses result in its metallization only after an incubation time that ranges from ∼150 ps to many nanoseconds, depending on the electric field strength. We show that these incubation times can be accounted for by purely thermal effects and that intrinsic electronic-switching mechanisms may only be revealed using larger electric fields at even shorter timescales. An important role is played by thermal effects in the electrically driven insulator-to-metal transition in V 2 O 3 .
ISSN:1748-3387
1748-3395
DOI:10.1038/nnano.2014.71