A simple and economic method for accurate determination of the energy peak efficiency of 208 keV γ-ray of 237U based on 241Pu/237U secular equilibrium

A new method is developed for the determination of energy peak efficiency of 208 keV γ-ray of 237 U based on 241 Pu/ 237 U secular equilibrium. Plutonium solution was purified to remove Am with Dowex 1 × 2 anion exchange chromatography and the concentration of 241 Pu in the purified solution was det...

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Veröffentlicht in:Journal of radioanalytical and nuclear chemistry 2014-03, Vol.299 (3), p.1987-1991
Hauptverfasser: Yi, Xiaowei, Yu, Gongshuo, Zhang, Jiamei, Zhang, Haitao, Li, Mei, Dang, Haijun
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container_end_page 1991
container_issue 3
container_start_page 1987
container_title Journal of radioanalytical and nuclear chemistry
container_volume 299
creator Yi, Xiaowei
Yu, Gongshuo
Zhang, Jiamei
Zhang, Haitao
Li, Mei
Dang, Haijun
description A new method is developed for the determination of energy peak efficiency of 208 keV γ-ray of 237 U based on 241 Pu/ 237 U secular equilibrium. Plutonium solution was purified to remove Am with Dowex 1 × 2 anion exchange chromatography and the concentration of 241 Pu in the purified solution was determined using 242 Pu isotope-dilution mass spectrometry on an inductively-coupled plasma mass spectrometry. The solution can be used as calibration source for the determination of energy peak efficiency of 208 keV γ-ray of 237 U after 48 days. The method was validated for a planar HPGe detector at the 12 mm above the detector surface. The results showed that this is a simple and economic method for determining the energy peak efficiency of gamma detectors for 208 keV γ-ray of 237 U.
doi_str_mv 10.1007/s10967-014-2937-0
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subjects Anion exchanging
Calibration
Chemistry
Chemistry and Materials Science
Detectors
Diagnostic Radiology
Economics
Energy (nuclear)
Energy management
Hadrons
Heavy Ions
Inorganic Chemistry
Mass spectrometry
Nuclear Chemistry
Nuclear Physics
Physical Chemistry
title A simple and economic method for accurate determination of the energy peak efficiency of 208 keV γ-ray of 237U based on 241Pu/237U secular equilibrium
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