Determination of ionization and tunneling times in high-order harmonic generation

From the numerical solution of the time-dependent Schrödinger equation, we obtain the times of ionization and return of the laser-driven electron in high-order harmonic generation by probing the dynamics with a second harmonic field polarized orthogonal to the fundamental field and observing the har...

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Veröffentlicht in:Physical review letters 2013-07, Vol.111 (4), p.043901-043901, Article 043901
Hauptverfasser: Zhao, Jing, Lein, Manfred
Format: Artikel
Sprache:eng
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Zusammenfassung:From the numerical solution of the time-dependent Schrödinger equation, we obtain the times of ionization and return of the laser-driven electron in high-order harmonic generation by probing the dynamics with a second harmonic field polarized orthogonal to the fundamental field and observing the harmonic emission in dependence on the two-color delay. Our retrieval method using complex-time evolution gives ionization and return times in excellent agreement with the quantum-orbit model, while a retrieval based on real-time classical dynamics can introduce substantial errors. Because of the imaginary parts, the harmonic signal polarized along the probe field is nonzero for any two-color delay. The tunneling time can be retrieved under an assumption for the return time.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.111.043901