Elastic electron scattering from water vapor and ice at high momentum transfer
We compare the area, peak separation, and width of the H and O elastic peak for light and heavy water, as observed in spectra of keV electrons scattered over large angles. Peak separation is well reproduced by the theory, but the O:H area ratio is somewhat larger than expected and is equal to the O:...
Gespeichert in:
Veröffentlicht in: | The Journal of chemical physics 2013-01, Vol.138 (4), p.044307-044307 |
---|---|
Hauptverfasser: | , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 044307 |
---|---|
container_issue | 4 |
container_start_page | 044307 |
container_title | The Journal of chemical physics |
container_volume | 138 |
creator | Vos, M Weigold, E Moreh, R |
description | We compare the area, peak separation, and width of the H and O elastic peak for light and heavy water, as observed in spectra of keV electrons scattered over large angles. Peak separation is well reproduced by the theory, but the O:H area ratio is somewhat larger than expected and is equal to the O:D area ratio. Thus no anomalous scattering from H was observed. Only minor differences are observed for scattering from a gaseous or a solid target. The extracted mean kinetic energy of H and D agreed within 5% with the calculated ones for ice. For the more difficult vapor measurements agreement was on a 12% level. A preliminary attempt to extract the O kinetic energy in ice agreed within 10% with the calculated values. |
doi_str_mv | 10.1063/1.4775810 |
format | Article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_miscellaneous_1323232937</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1323232937</sourcerecordid><originalsourceid>FETCH-LOGICAL-c419t-f97d566123a26449ec6982dae34f9cd02965b67673f45d5121ef9ee2edde8b483</originalsourceid><addsrcrecordid>eNqFkDtPwzAUhS0EoqEw8AeQRxhS_Iodj6gqD6mCBebIta_boDyK7YD496RqYUVnuDrSd8_wIXRJyYwSyW_pTChVlJQcoYySUudKanKMMkIYzbUkcoLOYnwnhFDFxCmaMM7L8UFk6HnRmJhqi6EBm0Lf4WhNShDqbo196Fv8ZcaGP822D9h0DtcWsEl4U683uO1b6NLQ4hRMFz2Ec3TiTRPh4nCn6O1-8Tp_zJcvD0_zu2VuBdUp91q5QkrKuGFSCA1W6pI5A1x4bR1hWhYrqaTiXhSuoIyC1wAMnINyJUo-Rdf73W3oPwaIqWrraKFpTAf9ECvK2S6aq_9RVhZCCqLZiN7sURv6GAP4ahvq1oTvipJqZ7qi1cH0yF4dZodVC-6P_FXLfwB0HHdQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1285464092</pqid></control><display><type>article</type><title>Elastic electron scattering from water vapor and ice at high momentum transfer</title><source>MEDLINE</source><source>AIP Journals Complete</source><source>AIP Digital Archive</source><source>Alma/SFX Local Collection</source><creator>Vos, M ; Weigold, E ; Moreh, R</creator><creatorcontrib>Vos, M ; Weigold, E ; Moreh, R</creatorcontrib><description>We compare the area, peak separation, and width of the H and O elastic peak for light and heavy water, as observed in spectra of keV electrons scattered over large angles. Peak separation is well reproduced by the theory, but the O:H area ratio is somewhat larger than expected and is equal to the O:D area ratio. Thus no anomalous scattering from H was observed. Only minor differences are observed for scattering from a gaseous or a solid target. The extracted mean kinetic energy of H and D agreed within 5% with the calculated ones for ice. For the more difficult vapor measurements agreement was on a 12% level. A preliminary attempt to extract the O kinetic energy in ice agreed within 10% with the calculated values.</description><identifier>ISSN: 0021-9606</identifier><identifier>EISSN: 1089-7690</identifier><identifier>DOI: 10.1063/1.4775810</identifier><identifier>PMID: 23387584</identifier><language>eng</language><publisher>United States</publisher><subject>Elasticity ; Electrons ; Ice ; Kinetics ; Steam</subject><ispartof>The Journal of chemical physics, 2013-01, Vol.138 (4), p.044307-044307</ispartof><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c419t-f97d566123a26449ec6982dae34f9cd02965b67673f45d5121ef9ee2edde8b483</citedby><cites>FETCH-LOGICAL-c419t-f97d566123a26449ec6982dae34f9cd02965b67673f45d5121ef9ee2edde8b483</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,776,780,27901,27902</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/23387584$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Vos, M</creatorcontrib><creatorcontrib>Weigold, E</creatorcontrib><creatorcontrib>Moreh, R</creatorcontrib><title>Elastic electron scattering from water vapor and ice at high momentum transfer</title><title>The Journal of chemical physics</title><addtitle>J Chem Phys</addtitle><description>We compare the area, peak separation, and width of the H and O elastic peak for light and heavy water, as observed in spectra of keV electrons scattered over large angles. Peak separation is well reproduced by the theory, but the O:H area ratio is somewhat larger than expected and is equal to the O:D area ratio. Thus no anomalous scattering from H was observed. Only minor differences are observed for scattering from a gaseous or a solid target. The extracted mean kinetic energy of H and D agreed within 5% with the calculated ones for ice. For the more difficult vapor measurements agreement was on a 12% level. A preliminary attempt to extract the O kinetic energy in ice agreed within 10% with the calculated values.</description><subject>Elasticity</subject><subject>Electrons</subject><subject>Ice</subject><subject>Kinetics</subject><subject>Steam</subject><issn>0021-9606</issn><issn>1089-7690</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2013</creationdate><recordtype>article</recordtype><sourceid>EIF</sourceid><recordid>eNqFkDtPwzAUhS0EoqEw8AeQRxhS_Iodj6gqD6mCBebIta_boDyK7YD496RqYUVnuDrSd8_wIXRJyYwSyW_pTChVlJQcoYySUudKanKMMkIYzbUkcoLOYnwnhFDFxCmaMM7L8UFk6HnRmJhqi6EBm0Lf4WhNShDqbo196Fv8ZcaGP822D9h0DtcWsEl4U683uO1b6NLQ4hRMFz2Ec3TiTRPh4nCn6O1-8Tp_zJcvD0_zu2VuBdUp91q5QkrKuGFSCA1W6pI5A1x4bR1hWhYrqaTiXhSuoIyC1wAMnINyJUo-Rdf73W3oPwaIqWrraKFpTAf9ECvK2S6aq_9RVhZCCqLZiN7sURv6GAP4ahvq1oTvipJqZ7qi1cH0yF4dZodVC-6P_FXLfwB0HHdQ</recordid><startdate>20130128</startdate><enddate>20130128</enddate><creator>Vos, M</creator><creator>Weigold, E</creator><creator>Moreh, R</creator><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7X8</scope><scope>7TG</scope><scope>KL.</scope></search><sort><creationdate>20130128</creationdate><title>Elastic electron scattering from water vapor and ice at high momentum transfer</title><author>Vos, M ; Weigold, E ; Moreh, R</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c419t-f97d566123a26449ec6982dae34f9cd02965b67673f45d5121ef9ee2edde8b483</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2013</creationdate><topic>Elasticity</topic><topic>Electrons</topic><topic>Ice</topic><topic>Kinetics</topic><topic>Steam</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Vos, M</creatorcontrib><creatorcontrib>Weigold, E</creatorcontrib><creatorcontrib>Moreh, R</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>MEDLINE - Academic</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><jtitle>The Journal of chemical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Vos, M</au><au>Weigold, E</au><au>Moreh, R</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Elastic electron scattering from water vapor and ice at high momentum transfer</atitle><jtitle>The Journal of chemical physics</jtitle><addtitle>J Chem Phys</addtitle><date>2013-01-28</date><risdate>2013</risdate><volume>138</volume><issue>4</issue><spage>044307</spage><epage>044307</epage><pages>044307-044307</pages><issn>0021-9606</issn><eissn>1089-7690</eissn><abstract>We compare the area, peak separation, and width of the H and O elastic peak for light and heavy water, as observed in spectra of keV electrons scattered over large angles. Peak separation is well reproduced by the theory, but the O:H area ratio is somewhat larger than expected and is equal to the O:D area ratio. Thus no anomalous scattering from H was observed. Only minor differences are observed for scattering from a gaseous or a solid target. The extracted mean kinetic energy of H and D agreed within 5% with the calculated ones for ice. For the more difficult vapor measurements agreement was on a 12% level. A preliminary attempt to extract the O kinetic energy in ice agreed within 10% with the calculated values.</abstract><cop>United States</cop><pmid>23387584</pmid><doi>10.1063/1.4775810</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
fulltext | fulltext |
identifier | ISSN: 0021-9606 |
ispartof | The Journal of chemical physics, 2013-01, Vol.138 (4), p.044307-044307 |
issn | 0021-9606 1089-7690 |
language | eng |
recordid | cdi_proquest_miscellaneous_1323232937 |
source | MEDLINE; AIP Journals Complete; AIP Digital Archive; Alma/SFX Local Collection |
subjects | Elasticity Electrons Ice Kinetics Steam |
title | Elastic electron scattering from water vapor and ice at high momentum transfer |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-09T00%3A25%3A31IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Elastic%20electron%20scattering%20from%20water%20vapor%20and%20ice%20at%20high%20momentum%20transfer&rft.jtitle=The%20Journal%20of%20chemical%20physics&rft.au=Vos,%20M&rft.date=2013-01-28&rft.volume=138&rft.issue=4&rft.spage=044307&rft.epage=044307&rft.pages=044307-044307&rft.issn=0021-9606&rft.eissn=1089-7690&rft_id=info:doi/10.1063/1.4775810&rft_dat=%3Cproquest_cross%3E1323232937%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=1285464092&rft_id=info:pmid/23387584&rfr_iscdi=true |