Structural and transport properties of epitaxial PrNiO3 thin films grown by molecular beam epitaxy

Epitaxial single crystal films of praseodymium nickelate (PrNiO3) have been grown by molecular beam epitaxy on LaAlO3(001) substrates. In-situ electron diffraction and ex-situ X-ray diffraction techniques confirm an epitaxial relationship to the underlying substrate. Crystalline quality depends stro...

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Veröffentlicht in:Journal of crystal growth 2013-03, Vol.366, p.51-54
Hauptverfasser: Feigl, L., Schultz, B.D., Ohya, S., Ouellette, D.G., Kozhanov, A., Palmstrøm, C.J.
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container_end_page 54
container_issue
container_start_page 51
container_title Journal of crystal growth
container_volume 366
creator Feigl, L.
Schultz, B.D.
Ohya, S.
Ouellette, D.G.
Kozhanov, A.
Palmstrøm, C.J.
description Epitaxial single crystal films of praseodymium nickelate (PrNiO3) have been grown by molecular beam epitaxy on LaAlO3(001) substrates. In-situ electron diffraction and ex-situ X-ray diffraction techniques confirm an epitaxial relationship to the underlying substrate. Crystalline quality depends strongly on the substrate temperature and activated oxygen flux during growth with the highest quality films formed at 600°C under high oxygen plasma fluxes. The metal–insulator transition for PrNiO3 films was suppressed as the crystalline quality of the layers was improved. ► Epitaxial single crystal films of PrNiO3 were grown by MBE on LaAlO3(001) substrates. ► Crystal quality depends strongly on substrate temperature and activated oxygen flux. ► Metal–insulator transition for PrNiO3 was suppressed as crystalline quality improved.
doi_str_mv 10.1016/j.jcrysgro.2012.12.018
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subjects A3. Molecular beam epitaxy
B1. Perovskites
B1. Rare earth nickelates
B2. Metal–insulator transition
Condensed matter: electronic structure, electrical, magnetic, and optical properties
Cross-disciplinary physics: materials science
rheology
Crystal growth
Crystal structure
Diffraction
Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures
Electronic transport phenomena in thin films and low-dimensional structures
Epitaxial growth
Exact sciences and technology
Flux
Fluxes
Materials science
Methods of deposition of films and coatings
film growth and epitaxy
Molecular beam epitaxy
Molecular, atomic, ion, and chemical beam epitaxy
Physics
Thin films
title Structural and transport properties of epitaxial PrNiO3 thin films grown by molecular beam epitaxy
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