Primary steps of electron and energy transfer in photosystem I: Effect of excitation pulse wavelength

Time-resolved differential spectra of photosystem I complex were obtained by the “pump-probe” technique with 25-fs pulses with maxima at 670, 700, and 720 nm. The ratio between the number of excited chlorophyll molecules of the antenna and of the reaction center was shown to depend on spectral chara...

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Veröffentlicht in:Biochemistry (Moscow) 2012-09, Vol.77 (9), p.1011-1020
Hauptverfasser: Semenov, A. Yu, Shelaev, I. V., Gostev, F. E., Mamedov, M. D., Shuvalov, V. A., Sarkisov, O. M., Nadtochenko, V. A.
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Sprache:eng
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Zusammenfassung:Time-resolved differential spectra of photosystem I complex were obtained by the “pump-probe” technique with 25-fs pulses with maxima at 670, 700, and 720 nm. The ratio between the number of excited chlorophyll molecules of the antenna and of the reaction center was shown to depend on spectral characteristics of the pump pulses. In all cases, an ultrafast (
ISSN:0006-2979
1608-3040
DOI:10.1134/S0006297912090088