Triplet-singlet conversion by broadband optical pumping
We demonstrate the conversion of cold Cs sub(2) molecules initially distributed over several vibrational levels of the lowest triplet state a super(3) capital sigma super(+) sub(u) into the singlet ground state X super(1) capital sigma super(+) sub(g). This conversion is realized by a broadband lase...
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Veröffentlicht in: | Physical review. A, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2012-03, Vol.85 (3), Article 030502 |
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Hauptverfasser: | , , , , , |
Format: | Artikel |
Sprache: | eng |
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Zusammenfassung: | We demonstrate the conversion of cold Cs sub(2) molecules initially distributed over several vibrational levels of the lowest triplet state a super(3) capital sigma super(+) sub(u) into the singlet ground state X super(1) capital sigma super(+) sub(g). This conversion is realized by a broadband laser exciting the molecules to a well-chosen state from which they may decay to the singlet state through two sequential single-photon emission steps: The first photon populates levels with mixed triplet-singlet character, making possible a second spontaneous emission down to several vibrational levels of the X super(1) capital sigma super(+) sub(g) states. By adding an optical scheme for vibrational cooling, a substantial fraction of molecules are transferred to the ground vibrational level of the singlet state. The efficiency of the conversion process, with and without vibrational cooling, is discussed at the end of the article. The presented conversion is general in scope and could be extended to other molecules. |
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ISSN: | 1050-2947 1094-1622 |
DOI: | 10.1103/PhysRevA.85.030502 |