Experimental gamma coincidence spectra recorded in prompt gamma neutron activation analysis

A feasibility study of gamma-gamma coincidence measurements in prompt gamma neutron activation analysis is carried out experimentally with a pulsed DT neutron generator, a polyethylene graphite cell and eight large NaI(Tl) scintillators. Detection limits are measured with multidimensional energy spe...

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Veröffentlicht in:J.Radioanal.Nucl.Chem 2024, Vol.333 (12), p.6577-6592
Hauptverfasser: Roult dit Rouaux, Jeremy, Carasco, Cedric, Loubet, Laurent, Perot, Bertrand, Tamagno, Leonie, Collot, Johann
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Sprache:eng
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Zusammenfassung:A feasibility study of gamma-gamma coincidence measurements in prompt gamma neutron activation analysis is carried out experimentally with a pulsed DT neutron generator, a polyethylene graphite cell and eight large NaI(Tl) scintillators. Detection limits are measured with multidimensional energy spectra created in gamma-gamma coincidence and compared to HPGe detector spectra. With a neutron emisison of 2.5 × 10 8 n.s −1 , the detection limit for sulfur is about 15 g in 20 min, while the detection limit is larger than 200 g when using the HPGe detector spectra. Processing the summ of up to three coincident gamma-ray energies highlights useful signal for a dysprosium sample, and allows for detecting permanent magnets containing 4% mass dysprosium within a rotor mock-up composed of stainless steel.
ISSN:0236-5731
1588-2780
DOI:10.1007/s10967-024-09822-x