Engineered g-C3N4/MnO2 Nanocomposite for Exceptional Photocatalytic Methylene Blue Degradation and Robust Antibacterial Impact

In this work, we reported the simple one-step wet impregnation method of g-C 3 N 4 /MnO 2 nanocomposites aimed at improving the photocatalytic degradation efficiency of methylene blue dye. The synthesized catalysts underwent comprehensive characterization using various techniques such as X-ray diffr...

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Veröffentlicht in:Journal of cluster science 2024-08, Vol.35 (6), p.1877-1887
Hauptverfasser: Krishnasamy, Mahalakshmi, Arumugam, Priyadharsan, Jayanthi, T. S., Choudhary, Shifali, Rojviroon, Thammasak, Matheswaran, Priyadharshini, Handayani, Murni, Periyasami, Govindasami, Diravidamani, Barathi, Rajendran, Ranjith
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Sprache:eng
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Zusammenfassung:In this work, we reported the simple one-step wet impregnation method of g-C 3 N 4 /MnO 2 nanocomposites aimed at improving the photocatalytic degradation efficiency of methylene blue dye. The synthesized catalysts underwent comprehensive characterization using various techniques such as X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FTIR), scanning electron microscopy (SEM), transmission electron microscopy (TEM), and ultraviolet-visible diffuse reflectance spectroscopy (UV-vis DRS) to investigate their physicochemical properties. Their photocatalytic performance was evaluated by the degradation of methylene blue (MB) dye under visible light irradiation. Consequently, the MnO 2 /g-C 3 N 4 nanocomposite demonstrates superior photocatalytic degradation performance compared to both bare MnO 2 and g-C 3 N 4 . This enhancement is attributed to the improved efficiency of charge carrier separation and interfacial charge transfer within the nanocomposite structure. The degradation efficiency of MnO 2 /g-C 3 N 4 nanocomposite was found 89% of MB under visible light irradiation at 120 min. Meanwhile, the recyclability analysis demonstrated that the MnO 2 /g-C 3 N 4 nanocomposite can be recycled four times. Furthermore, the substance demonstrated positive antibacterial activity against Escherichia coli , and Staphylococcus aureus bacterial strains. These findings suggest that the MnO 2 /g-C 3 N 4 nanocomposite, with its dual roles as a photocatalyst and an antibacterial agent, has potential applications in environmental decontamination.
ISSN:1040-7278
1572-8862
DOI:10.1007/s10876-024-02628-7