Unleashing the potentiality of metals: synergistic catalysis with light and electricity
The integration of transition metals as catalysts has opened new avenues for organic synthesis, including the activation and formation of diverse bonds. The combination of metal catalysis with photochemistry or electrochemistry has demonstrated enhanced reaction selectivity and reduced reliance on c...
Gespeichert in:
Veröffentlicht in: | Organic Chemistry Frontiers 2024-07, Vol.11 (14), p.4024-4040 |
---|---|
Hauptverfasser: | , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | 4040 |
---|---|
container_issue | 14 |
container_start_page | 4024 |
container_title | Organic Chemistry Frontiers |
container_volume | 11 |
creator | Shen, Zhengjia Tu, Jia-Lin Huang, Binbin |
description | The integration of transition metals as catalysts has opened new avenues for organic synthesis, including the activation and formation of diverse bonds. The combination of metal catalysis with photochemistry or electrochemistry has demonstrated enhanced reaction selectivity and reduced reliance on chemical oxidants. By harnessing the potential of organic photo-electrocatalysis, which combines photocatalysis with electrocatalysis, a wide range of efficient, selective and sustainable synthetic transformations have been achieved. This review provides a comprehensive overview of metal catalysis in photo-electrochemical systems, discussing reaction mechanisms and offering prospects for this triadic catalytic mode. |
doi_str_mv | 10.1039/D4QO00797B |
format | Article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_3076926866</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>3076926866</sourcerecordid><originalsourceid>FETCH-LOGICAL-c240t-4f478a71d57becaee6590ad3bf8142ba0e602f296af4cd4d8d17dcf864c01e0c3</originalsourceid><addsrcrecordid>eNpNUFtLwzAYDaLg0L34CwK-CdUvaZq0vum8wmAIDh9LlnxZM7p2JhnSf29lgj6dw-Fc4BByweCaQV7dPIi3BYCq1P0RmXAoeCYYr47_8VMyjXEDAIwXEgo1IR_LrkUdG9-taWqQ7vqEXfK69WmgvaNbTLqNtzQOHYa1j8kbavSoDdFH-uVTQ1u_bhLVnaXYoknBmzF7Tk7cGMTpL56R5dPj--wlmy-eX2d388xwASkTTqhSK2YLtUKjEWVRgbb5ypVM8JUGlMAdr6R2wlhhS8uUNa6UwgBDMPkZuTz07kL_uceY6k2_D904WeegZMVlKeXoujq4TOhjDOjqXfBbHYaaQf3zXf33Xf4N6sximQ</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>3076926866</pqid></control><display><type>article</type><title>Unleashing the potentiality of metals: synergistic catalysis with light and electricity</title><source>Royal Society Of Chemistry Journals 2008-</source><creator>Shen, Zhengjia ; Tu, Jia-Lin ; Huang, Binbin</creator><creatorcontrib>Shen, Zhengjia ; Tu, Jia-Lin ; Huang, Binbin</creatorcontrib><description>The integration of transition metals as catalysts has opened new avenues for organic synthesis, including the activation and formation of diverse bonds. The combination of metal catalysis with photochemistry or electrochemistry has demonstrated enhanced reaction selectivity and reduced reliance on chemical oxidants. By harnessing the potential of organic photo-electrocatalysis, which combines photocatalysis with electrocatalysis, a wide range of efficient, selective and sustainable synthetic transformations have been achieved. This review provides a comprehensive overview of metal catalysis in photo-electrochemical systems, discussing reaction mechanisms and offering prospects for this triadic catalytic mode.</description><identifier>ISSN: 2052-4129</identifier><identifier>ISSN: 2052-4110</identifier><identifier>EISSN: 2052-4129</identifier><identifier>EISSN: 2052-4110</identifier><identifier>DOI: 10.1039/D4QO00797B</identifier><language>eng</language><publisher>London: Royal Society of Chemistry</publisher><subject>Catalysis ; Catalysts ; Electrocatalysis ; Electrochemistry ; Metals ; Oxidants ; Oxidizing agents ; Photochemistry ; Reaction mechanisms ; Transition metals</subject><ispartof>Organic Chemistry Frontiers, 2024-07, Vol.11 (14), p.4024-4040</ispartof><rights>Copyright Royal Society of Chemistry 2024</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c240t-4f478a71d57becaee6590ad3bf8142ba0e602f296af4cd4d8d17dcf864c01e0c3</cites><orcidid>0009-0000-2553-8374 ; 0000-0002-2681-5537 ; 0000-0002-9205-0878</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,778,782,27907,27908</link.rule.ids></links><search><creatorcontrib>Shen, Zhengjia</creatorcontrib><creatorcontrib>Tu, Jia-Lin</creatorcontrib><creatorcontrib>Huang, Binbin</creatorcontrib><title>Unleashing the potentiality of metals: synergistic catalysis with light and electricity</title><title>Organic Chemistry Frontiers</title><description>The integration of transition metals as catalysts has opened new avenues for organic synthesis, including the activation and formation of diverse bonds. The combination of metal catalysis with photochemistry or electrochemistry has demonstrated enhanced reaction selectivity and reduced reliance on chemical oxidants. By harnessing the potential of organic photo-electrocatalysis, which combines photocatalysis with electrocatalysis, a wide range of efficient, selective and sustainable synthetic transformations have been achieved. This review provides a comprehensive overview of metal catalysis in photo-electrochemical systems, discussing reaction mechanisms and offering prospects for this triadic catalytic mode.</description><subject>Catalysis</subject><subject>Catalysts</subject><subject>Electrocatalysis</subject><subject>Electrochemistry</subject><subject>Metals</subject><subject>Oxidants</subject><subject>Oxidizing agents</subject><subject>Photochemistry</subject><subject>Reaction mechanisms</subject><subject>Transition metals</subject><issn>2052-4129</issn><issn>2052-4110</issn><issn>2052-4129</issn><issn>2052-4110</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNpNUFtLwzAYDaLg0L34CwK-CdUvaZq0vum8wmAIDh9LlnxZM7p2JhnSf29lgj6dw-Fc4BByweCaQV7dPIi3BYCq1P0RmXAoeCYYr47_8VMyjXEDAIwXEgo1IR_LrkUdG9-taWqQ7vqEXfK69WmgvaNbTLqNtzQOHYa1j8kbavSoDdFH-uVTQ1u_bhLVnaXYoknBmzF7Tk7cGMTpL56R5dPj--wlmy-eX2d388xwASkTTqhSK2YLtUKjEWVRgbb5ypVM8JUGlMAdr6R2wlhhS8uUNa6UwgBDMPkZuTz07kL_uceY6k2_D904WeegZMVlKeXoujq4TOhjDOjqXfBbHYaaQf3zXf33Xf4N6sximQ</recordid><startdate>20240709</startdate><enddate>20240709</enddate><creator>Shen, Zhengjia</creator><creator>Tu, Jia-Lin</creator><creator>Huang, Binbin</creator><general>Royal Society of Chemistry</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7QO</scope><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>FR3</scope><scope>JG9</scope><scope>P64</scope><orcidid>https://orcid.org/0009-0000-2553-8374</orcidid><orcidid>https://orcid.org/0000-0002-2681-5537</orcidid><orcidid>https://orcid.org/0000-0002-9205-0878</orcidid></search><sort><creationdate>20240709</creationdate><title>Unleashing the potentiality of metals: synergistic catalysis with light and electricity</title><author>Shen, Zhengjia ; Tu, Jia-Lin ; Huang, Binbin</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c240t-4f478a71d57becaee6590ad3bf8142ba0e602f296af4cd4d8d17dcf864c01e0c3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Catalysis</topic><topic>Catalysts</topic><topic>Electrocatalysis</topic><topic>Electrochemistry</topic><topic>Metals</topic><topic>Oxidants</topic><topic>Oxidizing agents</topic><topic>Photochemistry</topic><topic>Reaction mechanisms</topic><topic>Transition metals</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Shen, Zhengjia</creatorcontrib><creatorcontrib>Tu, Jia-Lin</creatorcontrib><creatorcontrib>Huang, Binbin</creatorcontrib><collection>CrossRef</collection><collection>Biotechnology Research Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Engineering Research Database</collection><collection>Materials Research Database</collection><collection>Biotechnology and BioEngineering Abstracts</collection><jtitle>Organic Chemistry Frontiers</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Shen, Zhengjia</au><au>Tu, Jia-Lin</au><au>Huang, Binbin</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Unleashing the potentiality of metals: synergistic catalysis with light and electricity</atitle><jtitle>Organic Chemistry Frontiers</jtitle><date>2024-07-09</date><risdate>2024</risdate><volume>11</volume><issue>14</issue><spage>4024</spage><epage>4040</epage><pages>4024-4040</pages><issn>2052-4129</issn><issn>2052-4110</issn><eissn>2052-4129</eissn><eissn>2052-4110</eissn><abstract>The integration of transition metals as catalysts has opened new avenues for organic synthesis, including the activation and formation of diverse bonds. The combination of metal catalysis with photochemistry or electrochemistry has demonstrated enhanced reaction selectivity and reduced reliance on chemical oxidants. By harnessing the potential of organic photo-electrocatalysis, which combines photocatalysis with electrocatalysis, a wide range of efficient, selective and sustainable synthetic transformations have been achieved. This review provides a comprehensive overview of metal catalysis in photo-electrochemical systems, discussing reaction mechanisms and offering prospects for this triadic catalytic mode.</abstract><cop>London</cop><pub>Royal Society of Chemistry</pub><doi>10.1039/D4QO00797B</doi><tpages>17</tpages><orcidid>https://orcid.org/0009-0000-2553-8374</orcidid><orcidid>https://orcid.org/0000-0002-2681-5537</orcidid><orcidid>https://orcid.org/0000-0002-9205-0878</orcidid></addata></record> |
fulltext | fulltext |
identifier | ISSN: 2052-4129 |
ispartof | Organic Chemistry Frontiers, 2024-07, Vol.11 (14), p.4024-4040 |
issn | 2052-4129 2052-4110 2052-4129 2052-4110 |
language | eng |
recordid | cdi_proquest_journals_3076926866 |
source | Royal Society Of Chemistry Journals 2008- |
subjects | Catalysis Catalysts Electrocatalysis Electrochemistry Metals Oxidants Oxidizing agents Photochemistry Reaction mechanisms Transition metals |
title | Unleashing the potentiality of metals: synergistic catalysis with light and electricity |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-16T22%3A56%3A43IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Unleashing%20the%20potentiality%20of%20metals:%20synergistic%20catalysis%20with%20light%20and%20electricity&rft.jtitle=Organic%20Chemistry%20Frontiers&rft.au=Shen,%20Zhengjia&rft.date=2024-07-09&rft.volume=11&rft.issue=14&rft.spage=4024&rft.epage=4040&rft.pages=4024-4040&rft.issn=2052-4129&rft.eissn=2052-4129&rft_id=info:doi/10.1039/D4QO00797B&rft_dat=%3Cproquest_cross%3E3076926866%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=3076926866&rft_id=info:pmid/&rfr_iscdi=true |