Selective diesel production from syngas over non-noble metal catalyst via a novel hydrogenolysis mechanism

Finite petroleum reserves and stringent environmental regulations stimulate the development of alternative fuels that are economically viable and clean. The diesel fuel (C10-20 hydrocarbons) derived from syngas by Fischer- Tropsch synthesis (FTS) is a promising choice, as it has the merits of low su...

Ausführliche Beschreibung

Gespeichert in:
Bibliographische Detailangaben
Veröffentlicht in:Science China. Chemistry 2015-06, Vol.58 (6), p.971-972
1. Verfasser: Qiao, Minghua
Format: Artikel
Sprache:eng
Schlagworte:
Online-Zugang:Volltext
Tags: Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
container_end_page 972
container_issue 6
container_start_page 971
container_title Science China. Chemistry
container_volume 58
creator Qiao, Minghua
description Finite petroleum reserves and stringent environmental regulations stimulate the development of alternative fuels that are economically viable and clean. The diesel fuel (C10-20 hydrocarbons) derived from syngas by Fischer- Tropsch synthesis (FTS) is a promising choice, as it has the merits of low sulfur and aronaatic contents, reduced NO, and particulate emissions, and high cetane number. Howev- er, the Anderson-Schulz-Flory (ASF) distribution imposes severe limitation on the selectivity towards diesel of only 39% over conventional FTS catalysts.
doi_str_mv 10.1007/s11426-015-5424-8
format Article
fullrecord <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2918655030</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><cqvip_id>664936178</cqvip_id><sourcerecordid>2918655030</sourcerecordid><originalsourceid>FETCH-LOGICAL-c365t-76afbdf170cfdc4018d679c2075d8dde3731d6250ee4864b608661b3c3d4289e3</originalsourceid><addsrcrecordid>eNp9kE1PwyAYxxujicvcB_BG9IxCoUCPZvEtWeJBPRMKT7suHWzQLdm3l2WL3uQAhOf_En5FcUvJAyVEPiZKeSkwoRWueMmxuigmVIkaUyXJZb4LybEsa3pdzFJakbwYI6WsJsXqEwawY78H5HpIMKBNDG6XX4JHbQxrlA6-MwmFPUTkg8c-NAOgNYxmQNbk_ZBGtO8NMnm8zwHLg4uhAx_ypE9ZaZfG92l9U1y1ZkgwO5_T4vvl-Wv-hhcfr-_zpwW2TFQjlsK0jWupJLZ1lhOqnJC1LYmsnHIOmGTUibIiAFwJ3giihKANs8zxUtXApsX9KTf_ZLuDNOpV2EWfK3VGoERVEUayip5UNoaUIrR6E_u1iQdNiT5S1SeqOlPVR6paZU958qSs9R3Ev-T_THfnomXw3Tb7fpuE4DUTVCr2A8fRhsc</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2918655030</pqid></control><display><type>article</type><title>Selective diesel production from syngas over non-noble metal catalyst via a novel hydrogenolysis mechanism</title><source>ProQuest Central Essentials</source><source>ProQuest Central (Alumni Edition)</source><source>ProQuest Central Student</source><source>ProQuest Central Korea</source><source>ProQuest Central UK/Ireland</source><source>Alma/SFX Local Collection</source><source>SpringerLink Journals - AutoHoldings</source><source>ProQuest Central</source><creator>Qiao, Minghua</creator><creatorcontrib>Qiao, Minghua</creatorcontrib><description>Finite petroleum reserves and stringent environmental regulations stimulate the development of alternative fuels that are economically viable and clean. The diesel fuel (C10-20 hydrocarbons) derived from syngas by Fischer- Tropsch synthesis (FTS) is a promising choice, as it has the merits of low sulfur and aronaatic contents, reduced NO, and particulate emissions, and high cetane number. Howev- er, the Anderson-Schulz-Flory (ASF) distribution imposes severe limitation on the selectivity towards diesel of only 39% over conventional FTS catalysts.</description><identifier>ISSN: 1674-7291</identifier><identifier>EISSN: 1869-1870</identifier><identifier>DOI: 10.1007/s11426-015-5424-8</identifier><language>eng</language><publisher>Beijing: Science China Press</publisher><subject>Chemistry ; Chemistry and Materials Science ; Chemistry/Food Science ; Highlights ; Hydrogenolysis ; Noble metals ; Synthesis gas ; 合成气 ; 替代燃料 ; 机制 ; 柴油燃料 ; 氢解 ; 生产 ; 非贵金属催化剂 ; 高十六烷值</subject><ispartof>Science China. Chemistry, 2015-06, Vol.58 (6), p.971-972</ispartof><rights>Science China Press and Springer-Verlag Berlin Heidelberg 2015</rights><rights>Science China Press and Springer-Verlag Berlin Heidelberg 2015.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c365t-76afbdf170cfdc4018d679c2075d8dde3731d6250ee4864b608661b3c3d4289e3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Uhttp://image.cqvip.com/vip1000/qk/60113X/60113X.jpg</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s11426-015-5424-8$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2918655030?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,780,784,21388,21389,21390,21391,23256,27924,27925,33530,33703,33744,34005,34314,41488,42557,43659,43787,43805,43953,44067,51319,64385,64389,72469</link.rule.ids></links><search><creatorcontrib>Qiao, Minghua</creatorcontrib><title>Selective diesel production from syngas over non-noble metal catalyst via a novel hydrogenolysis mechanism</title><title>Science China. Chemistry</title><addtitle>Sci. China Chem</addtitle><addtitle>SCIENCE CHINA Chemistry</addtitle><description>Finite petroleum reserves and stringent environmental regulations stimulate the development of alternative fuels that are economically viable and clean. The diesel fuel (C10-20 hydrocarbons) derived from syngas by Fischer- Tropsch synthesis (FTS) is a promising choice, as it has the merits of low sulfur and aronaatic contents, reduced NO, and particulate emissions, and high cetane number. Howev- er, the Anderson-Schulz-Flory (ASF) distribution imposes severe limitation on the selectivity towards diesel of only 39% over conventional FTS catalysts.</description><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Chemistry/Food Science</subject><subject>Highlights</subject><subject>Hydrogenolysis</subject><subject>Noble metals</subject><subject>Synthesis gas</subject><subject>合成气</subject><subject>替代燃料</subject><subject>机制</subject><subject>柴油燃料</subject><subject>氢解</subject><subject>生产</subject><subject>非贵金属催化剂</subject><subject>高十六烷值</subject><issn>1674-7291</issn><issn>1869-1870</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2015</creationdate><recordtype>article</recordtype><sourceid>ABUWG</sourceid><sourceid>AFKRA</sourceid><sourceid>AZQEC</sourceid><sourceid>BENPR</sourceid><sourceid>CCPQU</sourceid><sourceid>DWQXO</sourceid><sourceid>GNUQQ</sourceid><recordid>eNp9kE1PwyAYxxujicvcB_BG9IxCoUCPZvEtWeJBPRMKT7suHWzQLdm3l2WL3uQAhOf_En5FcUvJAyVEPiZKeSkwoRWueMmxuigmVIkaUyXJZb4LybEsa3pdzFJakbwYI6WsJsXqEwawY78H5HpIMKBNDG6XX4JHbQxrlA6-MwmFPUTkg8c-NAOgNYxmQNbk_ZBGtO8NMnm8zwHLg4uhAx_ypE9ZaZfG92l9U1y1ZkgwO5_T4vvl-Wv-hhcfr-_zpwW2TFQjlsK0jWupJLZ1lhOqnJC1LYmsnHIOmGTUibIiAFwJ3giihKANs8zxUtXApsX9KTf_ZLuDNOpV2EWfK3VGoERVEUayip5UNoaUIrR6E_u1iQdNiT5S1SeqOlPVR6paZU958qSs9R3Ev-T_THfnomXw3Tb7fpuE4DUTVCr2A8fRhsc</recordid><startdate>20150601</startdate><enddate>20150601</enddate><creator>Qiao, Minghua</creator><general>Science China Press</general><general>Springer Nature B.V</general><scope>2RA</scope><scope>92L</scope><scope>CQIGP</scope><scope>~WA</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7XB</scope><scope>88I</scope><scope>8FE</scope><scope>8FG</scope><scope>8FK</scope><scope>ABJCF</scope><scope>ABUWG</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BENPR</scope><scope>BGLVJ</scope><scope>CCPQU</scope><scope>D1I</scope><scope>DWQXO</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>KB.</scope><scope>M2P</scope><scope>PDBOC</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>PRINS</scope><scope>Q9U</scope></search><sort><creationdate>20150601</creationdate><title>Selective diesel production from syngas over non-noble metal catalyst via a novel hydrogenolysis mechanism</title><author>Qiao, Minghua</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c365t-76afbdf170cfdc4018d679c2075d8dde3731d6250ee4864b608661b3c3d4289e3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2015</creationdate><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Chemistry/Food Science</topic><topic>Highlights</topic><topic>Hydrogenolysis</topic><topic>Noble metals</topic><topic>Synthesis gas</topic><topic>合成气</topic><topic>替代燃料</topic><topic>机制</topic><topic>柴油燃料</topic><topic>氢解</topic><topic>生产</topic><topic>非贵金属催化剂</topic><topic>高十六烷值</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Qiao, Minghua</creatorcontrib><collection>中文科技期刊数据库</collection><collection>中文科技期刊数据库-CALIS站点</collection><collection>中文科技期刊数据库-7.0平台</collection><collection>中文科技期刊数据库- 镜像站点</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Technology Collection</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>Materials Science &amp; Engineering Collection</collection><collection>ProQuest Central (Alumni Edition)</collection><collection>ProQuest Central UK/Ireland</collection><collection>ProQuest Central Essentials</collection><collection>ProQuest Central</collection><collection>Technology Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Materials Science Collection</collection><collection>ProQuest Central Korea</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>Materials Science Database</collection><collection>Science Database</collection><collection>Materials Science Collection</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central China</collection><collection>ProQuest Central Basic</collection><jtitle>Science China. Chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Qiao, Minghua</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Selective diesel production from syngas over non-noble metal catalyst via a novel hydrogenolysis mechanism</atitle><jtitle>Science China. Chemistry</jtitle><stitle>Sci. China Chem</stitle><addtitle>SCIENCE CHINA Chemistry</addtitle><date>2015-06-01</date><risdate>2015</risdate><volume>58</volume><issue>6</issue><spage>971</spage><epage>972</epage><pages>971-972</pages><issn>1674-7291</issn><eissn>1869-1870</eissn><abstract>Finite petroleum reserves and stringent environmental regulations stimulate the development of alternative fuels that are economically viable and clean. The diesel fuel (C10-20 hydrocarbons) derived from syngas by Fischer- Tropsch synthesis (FTS) is a promising choice, as it has the merits of low sulfur and aronaatic contents, reduced NO, and particulate emissions, and high cetane number. Howev- er, the Anderson-Schulz-Flory (ASF) distribution imposes severe limitation on the selectivity towards diesel of only 39% over conventional FTS catalysts.</abstract><cop>Beijing</cop><pub>Science China Press</pub><doi>10.1007/s11426-015-5424-8</doi><tpages>2</tpages></addata></record>
fulltext fulltext
identifier ISSN: 1674-7291
ispartof Science China. Chemistry, 2015-06, Vol.58 (6), p.971-972
issn 1674-7291
1869-1870
language eng
recordid cdi_proquest_journals_2918655030
source ProQuest Central Essentials; ProQuest Central (Alumni Edition); ProQuest Central Student; ProQuest Central Korea; ProQuest Central UK/Ireland; Alma/SFX Local Collection; SpringerLink Journals - AutoHoldings; ProQuest Central
subjects Chemistry
Chemistry and Materials Science
Chemistry/Food Science
Highlights
Hydrogenolysis
Noble metals
Synthesis gas
合成气
替代燃料
机制
柴油燃料
氢解
生产
非贵金属催化剂
高十六烷值
title Selective diesel production from syngas over non-noble metal catalyst via a novel hydrogenolysis mechanism
url https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-05T21%3A04%3A51IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Selective%20diesel%20production%20from%20syngas%20over%20non-noble%20metal%20catalyst%20via%20a%20novel%20hydrogenolysis%20mechanism&rft.jtitle=Science%20China.%20Chemistry&rft.au=Qiao,%20Minghua&rft.date=2015-06-01&rft.volume=58&rft.issue=6&rft.spage=971&rft.epage=972&rft.pages=971-972&rft.issn=1674-7291&rft.eissn=1869-1870&rft_id=info:doi/10.1007/s11426-015-5424-8&rft_dat=%3Cproquest_cross%3E2918655030%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2918655030&rft_id=info:pmid/&rft_cqvip_id=664936178&rfr_iscdi=true