A diatomite-derived N-doped carbon aerogel with 98% sulfur loading for the enhancement of Li-S battery performance

Improving the sulfur content and cycling performance of the cathode is the key to the commercial application of lithium-sulfur batteries. Herein, the diatomite-derived nitrogen-doped carbon aerogel provides an ample sulfur loading space that can be loaded with 98% sublimated sulfur. The Li-S battery...

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Veröffentlicht in:New journal of chemistry 2023-03, Vol.47 (1), p.4614-4618
Hauptverfasser: Jiang, Zhiyi, Zhang, Shilin, Dong, Xiongbo, Xu, Zonglin, Sarwar, Muhammad Tariq, Yan, Chenyu, Yang, Caihong, Tang, Aidong, Yang, Huming
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Sprache:eng
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Zusammenfassung:Improving the sulfur content and cycling performance of the cathode is the key to the commercial application of lithium-sulfur batteries. Herein, the diatomite-derived nitrogen-doped carbon aerogel provides an ample sulfur loading space that can be loaded with 98% sublimated sulfur. The Li-S battery delivered an initial discharge capacity of 703.1 mAh g −1 and still retained 510.1 mAh g −1 at 0.5C after 200 cycles, which is attributed to the highly disordered carbon and catalytic activity. The ultralight carbon material with diatomite as template can drive 98 wt% sulfur material with only 2 wt%, and it still has high performance when used as the cathode material for lithium sulfur batteries.
ISSN:1144-0546
1369-9261
DOI:10.1039/d2nj05444b