Unveiling the Protonation Kinetics‐Dependent Selectivity in Nitrogen Electroreduction: Achieving 75.05 % Selectivity

While higher selectivity of nitrogen reduction reaction (NRR) to ammonia (NH3) is always achieved in alkali, the selectivity dependence on nitrogen (N2) protonation and mechanisms therein are unrevealed. Herein, we profile how the NRR selectivity theoretically relies upon the first protonation that...

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Veröffentlicht in:	Angewandte Chemie International Edition 2022-12, Vol.61 (50), p.n/a
Hauptverfasser:	Liu, Yang, Wang, Lingling, Chen, Lin, Wang, Hongdan, Jadhav, Amol R., Yang, Taehun, Wang, Yixuan, Zhang, Jinqiang, Kumar, Ashwani, Lee, Jinsun, Bui, Viet Q., Kim, Min Gyu, Lee, Hyoyoung
Format:	Artikel
Sprache:	eng
Schlagworte:	Adjustable Protonation Kinetics Ammonia Catalysts Chemical reduction Copper Electrochemical impedance spectroscopy Electrochemistry Electronic Modulation Infrared spectroscopy Intermediates Kinetics Modulators Nitrogen Nitrogen Electroreduction Nitrogenase Operando Electrochemical Impedance Spectroscopy Simulations Protonation Protonation-Selectivity Relation Raman spectroscopy Selectivity Spectroscopy Zinc
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