Synthesis and characterization of ytterbium oxide: A novel CMAS‐resistant environmental barrier coating material
Demand for more powerful aircraft promotes development of ceramic matrix composites and environmental barrier coating (EBC). A promising EBC material, ytterbium oxide (Yb2O3), was fabricated by hot pressing, and its properties were systemically investigated. The evaluation of thermal properties prov...
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| Veröffentlicht in: | Journal of the American Ceramic Society 2023-01, Vol.106 (1), p.621-631 |
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| creator | Zhang, Guangheng Zhang, Jie Wang, Jingyang |
| description | Demand for more powerful aircraft promotes development of ceramic matrix composites and environmental barrier coating (EBC). A promising EBC material, ytterbium oxide (Yb2O3), was fabricated by hot pressing, and its properties were systemically investigated. The evaluation of thermal properties provides a baseline for the application of Yb2O3 on SiCf/SiC or Al2O3f/Al2O3 composites. The performance in water vapor and molten calcium–magnesium–aluminosilicate (CMAS) environments indicates its excellent durability in harsh environment. Compared with rare‐earth silicates, the thermochemical interactions between ytterbium oxide and CMAS changed greatly with the absence of silicon oxide. Reactions of ytterbium oxide with CMAS form several reaction products, including apatite, garnet, and silicocarnotite. The crystallization of garnet and silicocarnotite could effectively consume and solidify the CMAS melt, which prevents the melt infiltration and mitigates the further corrosion. |
| doi_str_mv | 10.1111/jace.18786 |
| format | Article |
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A promising EBC material, ytterbium oxide (Yb2O3), was fabricated by hot pressing, and its properties were systemically investigated. The evaluation of thermal properties provides a baseline for the application of Yb2O3 on SiCf/SiC or Al2O3f/Al2O3 composites. The performance in water vapor and molten calcium–magnesium–aluminosilicate (CMAS) environments indicates its excellent durability in harsh environment. Compared with rare‐earth silicates, the thermochemical interactions between ytterbium oxide and CMAS changed greatly with the absence of silicon oxide. Reactions of ytterbium oxide with CMAS form several reaction products, including apatite, garnet, and silicocarnotite. The crystallization of garnet and silicocarnotite could effectively consume and solidify the CMAS melt, which prevents the melt infiltration and mitigates the further corrosion.</description><identifier>ISSN: 0002-7820</identifier><identifier>EISSN: 1551-2916</identifier><identifier>DOI: 10.1111/jace.18786</identifier><language>eng</language><publisher>Columbus: Wiley Subscription Services, Inc</publisher><subject>Aluminosilicates ; Aluminum oxide ; Aluminum silicates ; Apatite ; Ceramic fiber reinforced ceramics ; Ceramic matrix composites ; CMAS resistant ; Crystallization ; environmental barrier coating ; Garnets ; Hot pressing ; Magnesium ; Reaction products ; Silicates ; Silicon carbide ; Silicon oxides ; thermal property ; Thermodynamic properties ; Water vapor ; water vapor corrosion ; Ytterbium ; ytterbium oxide</subject><ispartof>Journal of the American Ceramic Society, 2023-01, Vol.106 (1), p.621-631</ispartof><rights>2022 The American Ceramic Society.</rights><rights>2023 The American Ceramic Society.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c2316-ce7c594d4f34a80e65da2abf3e6daeb218c36029964e372c96c89721088b42da3</citedby><cites>FETCH-LOGICAL-c2316-ce7c594d4f34a80e65da2abf3e6daeb218c36029964e372c96c89721088b42da3</cites><orcidid>0000-0002-1919-3602 ; 0000-0002-4748-8512</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1111%2Fjace.18786$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1111%2Fjace.18786$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,776,780,1411,27903,27904,45553,45554</link.rule.ids></links><search><creatorcontrib>Zhang, Guangheng</creatorcontrib><creatorcontrib>Zhang, Jie</creatorcontrib><creatorcontrib>Wang, Jingyang</creatorcontrib><title>Synthesis and characterization of ytterbium oxide: A novel CMAS‐resistant environmental barrier coating material</title><title>Journal of the American Ceramic Society</title><description>Demand for more powerful aircraft promotes development of ceramic matrix composites and environmental barrier coating (EBC). A promising EBC material, ytterbium oxide (Yb2O3), was fabricated by hot pressing, and its properties were systemically investigated. The evaluation of thermal properties provides a baseline for the application of Yb2O3 on SiCf/SiC or Al2O3f/Al2O3 composites. The performance in water vapor and molten calcium–magnesium–aluminosilicate (CMAS) environments indicates its excellent durability in harsh environment. Compared with rare‐earth silicates, the thermochemical interactions between ytterbium oxide and CMAS changed greatly with the absence of silicon oxide. Reactions of ytterbium oxide with CMAS form several reaction products, including apatite, garnet, and silicocarnotite. The crystallization of garnet and silicocarnotite could effectively consume and solidify the CMAS melt, which prevents the melt infiltration and mitigates the further corrosion.</description><subject>Aluminosilicates</subject><subject>Aluminum oxide</subject><subject>Aluminum silicates</subject><subject>Apatite</subject><subject>Ceramic fiber reinforced ceramics</subject><subject>Ceramic matrix composites</subject><subject>CMAS resistant</subject><subject>Crystallization</subject><subject>environmental barrier coating</subject><subject>Garnets</subject><subject>Hot pressing</subject><subject>Magnesium</subject><subject>Reaction products</subject><subject>Silicates</subject><subject>Silicon carbide</subject><subject>Silicon oxides</subject><subject>thermal property</subject><subject>Thermodynamic properties</subject><subject>Water vapor</subject><subject>water vapor corrosion</subject><subject>Ytterbium</subject><subject>ytterbium oxide</subject><issn>0002-7820</issn><issn>1551-2916</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2023</creationdate><recordtype>article</recordtype><recordid>eNp9kM1OwzAQhC0EEqVw4QkscUNKsZ00sblFFb8q4lA4WxtnQ10ldnHSQjnxCDwjT0JKObOX0UjfzEpDyClnI97fxQIMjrjMZLpHBnw85pFQPN0nA8aYiDIp2CE5attFb7mSyYCE2cZ1c2xtS8GV1MwhgOkw2A_orHfUV3TT9b6wq4b6d1viJc2p82us6eQhn31_foVtugPXUXRrG7xr0HVQ0wJCsBio8X2Ve6ENbHuhPiYHFdQtnvzpkDxfXz1NbqPp483dJJ9GRsQ8jQxmZqySMqniBCTDdFyCgKKKMS0BC8GliVMmlEoTjDNhVGqkygRnUhaJKCEekrNd7zL41xW2nV74VXD9Sy2ymEnFVSZ76nxHmeDbNmCll8E2EDaaM73dVG831b-b9jDfwW-2xs0_pL7PJ1e7zA81JnwH</recordid><startdate>202301</startdate><enddate>202301</enddate><creator>Zhang, Guangheng</creator><creator>Zhang, Jie</creator><creator>Wang, Jingyang</creator><general>Wiley Subscription Services, Inc</general><scope>AAYXX</scope><scope>CITATION</scope><scope>7QQ</scope><scope>7SR</scope><scope>8FD</scope><scope>JG9</scope><orcidid>https://orcid.org/0000-0002-1919-3602</orcidid><orcidid>https://orcid.org/0000-0002-4748-8512</orcidid></search><sort><creationdate>202301</creationdate><title>Synthesis and characterization of ytterbium oxide: A novel CMAS‐resistant environmental barrier coating material</title><author>Zhang, Guangheng ; Zhang, Jie ; Wang, Jingyang</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c2316-ce7c594d4f34a80e65da2abf3e6daeb218c36029964e372c96c89721088b42da3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2023</creationdate><topic>Aluminosilicates</topic><topic>Aluminum oxide</topic><topic>Aluminum silicates</topic><topic>Apatite</topic><topic>Ceramic fiber reinforced ceramics</topic><topic>Ceramic matrix composites</topic><topic>CMAS resistant</topic><topic>Crystallization</topic><topic>environmental barrier coating</topic><topic>Garnets</topic><topic>Hot pressing</topic><topic>Magnesium</topic><topic>Reaction products</topic><topic>Silicates</topic><topic>Silicon carbide</topic><topic>Silicon oxides</topic><topic>thermal property</topic><topic>Thermodynamic properties</topic><topic>Water vapor</topic><topic>water vapor corrosion</topic><topic>Ytterbium</topic><topic>ytterbium oxide</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhang, Guangheng</creatorcontrib><creatorcontrib>Zhang, Jie</creatorcontrib><creatorcontrib>Wang, Jingyang</creatorcontrib><collection>CrossRef</collection><collection>Ceramic Abstracts</collection><collection>Engineered Materials Abstracts</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><jtitle>Journal of the American Ceramic Society</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zhang, Guangheng</au><au>Zhang, Jie</au><au>Wang, Jingyang</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synthesis and characterization of ytterbium oxide: A novel CMAS‐resistant environmental barrier coating material</atitle><jtitle>Journal of the American Ceramic Society</jtitle><date>2023-01</date><risdate>2023</risdate><volume>106</volume><issue>1</issue><spage>621</spage><epage>631</epage><pages>621-631</pages><issn>0002-7820</issn><eissn>1551-2916</eissn><abstract>Demand for more powerful aircraft promotes development of ceramic matrix composites and environmental barrier coating (EBC). A promising EBC material, ytterbium oxide (Yb2O3), was fabricated by hot pressing, and its properties were systemically investigated. The evaluation of thermal properties provides a baseline for the application of Yb2O3 on SiCf/SiC or Al2O3f/Al2O3 composites. The performance in water vapor and molten calcium–magnesium–aluminosilicate (CMAS) environments indicates its excellent durability in harsh environment. Compared with rare‐earth silicates, the thermochemical interactions between ytterbium oxide and CMAS changed greatly with the absence of silicon oxide. Reactions of ytterbium oxide with CMAS form several reaction products, including apatite, garnet, and silicocarnotite. The crystallization of garnet and silicocarnotite could effectively consume and solidify the CMAS melt, which prevents the melt infiltration and mitigates the further corrosion.</abstract><cop>Columbus</cop><pub>Wiley Subscription Services, Inc</pub><doi>10.1111/jace.18786</doi><tpages>11</tpages><orcidid>https://orcid.org/0000-0002-1919-3602</orcidid><orcidid>https://orcid.org/0000-0002-4748-8512</orcidid></addata></record> |
| fulltext | fulltext |
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| ispartof | Journal of the American Ceramic Society, 2023-01, Vol.106 (1), p.621-631 |
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| language | eng |
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| source | Wiley Online Library Journals Frontfile Complete |
| subjects | Aluminosilicates Aluminum oxide Aluminum silicates Apatite Ceramic fiber reinforced ceramics Ceramic matrix composites CMAS resistant Crystallization environmental barrier coating Garnets Hot pressing Magnesium Reaction products Silicates Silicon carbide Silicon oxides thermal property Thermodynamic properties Water vapor water vapor corrosion Ytterbium ytterbium oxide |
| title | Synthesis and characterization of ytterbium oxide: A novel CMAS‐resistant environmental barrier coating material |
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