Removal of malachite green by electrochemical oxidation polymerization and electrochemical reduction precipitation: its kinetics and intermediates
In this paper, removal of malachite green (MG) by two separate processes, namely electrochemical oxidization polymerization and electrochemical reduction precipitation process, was studied. Reaction rate constants ( k 0 ), exchange current density i 0 , the transfer coefficients β and the diffusion...
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| Veröffentlicht in: | Journal of solid state electrochemistry 2022-10, Vol.26 (10), p.2231-2246 |
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| container_title | Journal of solid state electrochemistry |
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| creator | Wang, Li Wang, Junbo Yu, Aishui Yu, Zuolong |
| description | In this paper, removal of malachite green (MG) by two separate processes, namely electrochemical oxidization polymerization and electrochemical reduction precipitation process, was studied. Reaction rate constants (
k
0
), exchange current density
i
0
, the transfer coefficients
β
and the diffusion coefficient
D
values were all tested. TR-FTIR (time-resolved Fourier transform infrared spectroscopy), UPLC-MS (ultra-performance liquid chromatography–mass spectrometry), and GC–MS (gas chromatography–mass spectrometer) analyses were applied to investigate the pathway and mechanism of MG degradation. The results show that both electrochemical oxidization polymerization and electrochemical reduction precipitation process were efficient to remove MG. |
| doi_str_mv | 10.1007/s10008-022-05242-7 |
| format | Article |
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k
0
), exchange current density
i
0
, the transfer coefficients
β
and the diffusion coefficient
D
values were all tested. TR-FTIR (time-resolved Fourier transform infrared spectroscopy), UPLC-MS (ultra-performance liquid chromatography–mass spectrometry), and GC–MS (gas chromatography–mass spectrometer) analyses were applied to investigate the pathway and mechanism of MG degradation. The results show that both electrochemical oxidization polymerization and electrochemical reduction precipitation process were efficient to remove MG.</description><identifier>ISSN: 1432-8488</identifier><identifier>EISSN: 1433-0768</identifier><identifier>DOI: 10.1007/s10008-022-05242-7</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Analytical Chemistry ; Characterization and Evaluation of Materials ; Chemical precipitation ; Chemical reduction ; Chemistry ; Chemistry and Materials Science ; Condensed Matter Physics ; Diffusion coefficient ; Electrochemical oxidation ; Electrochemistry ; Energy Storage ; Fourier transforms ; Gas chromatography ; Liquid chromatography ; Malachite green ; Mass spectrometry ; Original Paper ; Physical Chemistry ; Polymerization ; Rate constants</subject><ispartof>Journal of solid state electrochemistry, 2022-10, Vol.26 (10), p.2231-2246</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c319t-ff2fd8b05859167b9d29031c9cd20e2df380b310763d9f72116912a2586550fe3</citedby><cites>FETCH-LOGICAL-c319t-ff2fd8b05859167b9d29031c9cd20e2df380b310763d9f72116912a2586550fe3</cites><orcidid>0000-0002-7555-3836</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1007/s10008-022-05242-7$$EPDF$$P50$$Gspringer$$H</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1007/s10008-022-05242-7$$EHTML$$P50$$Gspringer$$H</linktohtml><link.rule.ids>314,776,780,27901,27902,41464,42533,51294</link.rule.ids></links><search><creatorcontrib>Wang, Li</creatorcontrib><creatorcontrib>Wang, Junbo</creatorcontrib><creatorcontrib>Yu, Aishui</creatorcontrib><creatorcontrib>Yu, Zuolong</creatorcontrib><title>Removal of malachite green by electrochemical oxidation polymerization and electrochemical reduction precipitation: its kinetics and intermediates</title><title>Journal of solid state electrochemistry</title><addtitle>J Solid State Electrochem</addtitle><description>In this paper, removal of malachite green (MG) by two separate processes, namely electrochemical oxidization polymerization and electrochemical reduction precipitation process, was studied. Reaction rate constants (
k
0
), exchange current density
i
0
, the transfer coefficients
β
and the diffusion coefficient
D
values were all tested. TR-FTIR (time-resolved Fourier transform infrared spectroscopy), UPLC-MS (ultra-performance liquid chromatography–mass spectrometry), and GC–MS (gas chromatography–mass spectrometer) analyses were applied to investigate the pathway and mechanism of MG degradation. The results show that both electrochemical oxidization polymerization and electrochemical reduction precipitation process were efficient to remove MG.</description><subject>Analytical Chemistry</subject><subject>Characterization and Evaluation of Materials</subject><subject>Chemical precipitation</subject><subject>Chemical reduction</subject><subject>Chemistry</subject><subject>Chemistry and Materials Science</subject><subject>Condensed Matter Physics</subject><subject>Diffusion coefficient</subject><subject>Electrochemical oxidation</subject><subject>Electrochemistry</subject><subject>Energy Storage</subject><subject>Fourier transforms</subject><subject>Gas chromatography</subject><subject>Liquid chromatography</subject><subject>Malachite green</subject><subject>Mass spectrometry</subject><subject>Original Paper</subject><subject>Physical Chemistry</subject><subject>Polymerization</subject><subject>Rate constants</subject><issn>1432-8488</issn><issn>1433-0768</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNp9kMtKAzEUhgdRsFZfwNWA69GTpDPJuBPxBgVBdB0yyUmbOjeTVKyP4RM77QguBDfnAt__H86fJKcEzgkAvwhDBZEBpRnkdEYzvpdMyIyxDHgh9nczzcRMiMPkKIQVAOEFgUny9YRN967qtLNpo2qlly5iuvCIbVptUqxRR9_pJTZOb6kPZ1R0XZv2Xb1p0LvPcVWt-QN7NGs9wh61613csZepiyF9dS1Gp8NO6dqIvkHjVMRwnBxYVQc8-enT5OX25vn6Pps_3j1cX80zzUgZM2upNaKCXOQlKXhVGloCI7rUhgJSY5mAipHhf2ZKyykhRUmoorko8hwssmlyNvr2vntbY4hy1a19O5yUlEPOORvqQNGR0r4LwaOVvXeN8htJQG6zl2P2cshe7rKXfBCxURQGuF2g_7X-R_UNzSSKYw</recordid><startdate>20221001</startdate><enddate>20221001</enddate><creator>Wang, Li</creator><creator>Wang, Junbo</creator><creator>Yu, Aishui</creator><creator>Yu, Zuolong</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-7555-3836</orcidid></search><sort><creationdate>20221001</creationdate><title>Removal of malachite green by electrochemical oxidation polymerization and electrochemical reduction precipitation: its kinetics and intermediates</title><author>Wang, Li ; Wang, Junbo ; Yu, Aishui ; Yu, Zuolong</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c319t-ff2fd8b05859167b9d29031c9cd20e2df380b310763d9f72116912a2586550fe3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Analytical Chemistry</topic><topic>Characterization and Evaluation of Materials</topic><topic>Chemical precipitation</topic><topic>Chemical reduction</topic><topic>Chemistry</topic><topic>Chemistry and Materials Science</topic><topic>Condensed Matter Physics</topic><topic>Diffusion coefficient</topic><topic>Electrochemical oxidation</topic><topic>Electrochemistry</topic><topic>Energy Storage</topic><topic>Fourier transforms</topic><topic>Gas chromatography</topic><topic>Liquid chromatography</topic><topic>Malachite green</topic><topic>Mass spectrometry</topic><topic>Original Paper</topic><topic>Physical Chemistry</topic><topic>Polymerization</topic><topic>Rate constants</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Li</creatorcontrib><creatorcontrib>Wang, Junbo</creatorcontrib><creatorcontrib>Yu, Aishui</creatorcontrib><creatorcontrib>Yu, Zuolong</creatorcontrib><collection>CrossRef</collection><jtitle>Journal of solid state electrochemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Li</au><au>Wang, Junbo</au><au>Yu, Aishui</au><au>Yu, Zuolong</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Removal of malachite green by electrochemical oxidation polymerization and electrochemical reduction precipitation: its kinetics and intermediates</atitle><jtitle>Journal of solid state electrochemistry</jtitle><stitle>J Solid State Electrochem</stitle><date>2022-10-01</date><risdate>2022</risdate><volume>26</volume><issue>10</issue><spage>2231</spage><epage>2246</epage><pages>2231-2246</pages><issn>1432-8488</issn><eissn>1433-0768</eissn><abstract>In this paper, removal of malachite green (MG) by two separate processes, namely electrochemical oxidization polymerization and electrochemical reduction precipitation process, was studied. Reaction rate constants (
k
0
), exchange current density
i
0
, the transfer coefficients
β
and the diffusion coefficient
D
values were all tested. TR-FTIR (time-resolved Fourier transform infrared spectroscopy), UPLC-MS (ultra-performance liquid chromatography–mass spectrometry), and GC–MS (gas chromatography–mass spectrometer) analyses were applied to investigate the pathway and mechanism of MG degradation. The results show that both electrochemical oxidization polymerization and electrochemical reduction precipitation process were efficient to remove MG.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1007/s10008-022-05242-7</doi><tpages>16</tpages><orcidid>https://orcid.org/0000-0002-7555-3836</orcidid></addata></record> |
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| subjects | Analytical Chemistry Characterization and Evaluation of Materials Chemical precipitation Chemical reduction Chemistry Chemistry and Materials Science Condensed Matter Physics Diffusion coefficient Electrochemical oxidation Electrochemistry Energy Storage Fourier transforms Gas chromatography Liquid chromatography Malachite green Mass spectrometry Original Paper Physical Chemistry Polymerization Rate constants |
| title | Removal of malachite green by electrochemical oxidation polymerization and electrochemical reduction precipitation: its kinetics and intermediates |
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