Relevance of nonadiabatic effects in TiOCl

We analyze the effect of the phonon dynamics on a recently proposed model for the uniform-incommensurate transition seen in TiOX compounds. The study is based on a recently developed formalism for nonadiabatic spin-Peierls systems based on bosonization and a mean field RPA approximation for the inte...

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Veröffentlicht in:Journal of physics. Conference series 2010-01, Vol.200 (2), p.022032
Hauptverfasser: Mastrogiuseppe, Diego, Dobry, Ariel
Format: Artikel
Sprache:eng
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Zusammenfassung:We analyze the effect of the phonon dynamics on a recently proposed model for the uniform-incommensurate transition seen in TiOX compounds. The study is based on a recently developed formalism for nonadiabatic spin-Peierls systems based on bosonization and a mean field RPA approximation for the interchain coupling. To reproduce the measured low temperature spin gap, a spin-phonon coupling quite bigger than the one predicted from an adiabatic approach is required. This high value is compatible with the renormalization of the phonons in the high temperature phase seen in inelastic x-ray experiments. Our theory accounts for the temperature of the incommensurate transition and the value of the incommensurate wave vector at the transition point.
ISSN:1742-6596
1742-6588
1742-6596
DOI:10.1088/1742-6596/200/2/022032