Linear dichroism in few-photon ionization of laser-dressed helium

Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay betw...

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Veröffentlicht in:The European physical journal. D, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2021-07, Vol.75 (7), Article 205
Hauptverfasser: Meister, Severin, Bondy, Aaron, Schnorr, Kirsten, Augustin, Sven, Lindenblatt, Hannes, Trost, Florian, Xie, Xinhua, Braune, Markus, Manschwetus, Bastian, Schirmel, Nora, Redlin, Harald, Douguet, Nicolas, Pfeifer, Thomas, Bartschat, Klaus, Moshammer, Robert
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container_title The European physical journal. D, Atomic, molecular, and optical physics
container_volume 75
creator Meister, Severin
Bondy, Aaron
Schnorr, Kirsten
Augustin, Sven
Lindenblatt, Hannes
Trost, Florian
Xie, Xinhua
Braune, Markus
Manschwetus, Bastian
Schirmel, Nora
Redlin, Harald
Douguet, Nicolas
Pfeifer, Thomas
Bartschat, Klaus
Moshammer, Robert
description Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation. Graphic abstract
doi_str_mv 10.1140/epjd/s10053-021-00218-0
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subjects Applications of Nonlinear Dynamics and Chaos Theory
Atomic
Dichroism
Excitation
Helium
Infrared radiation
Ionization
Lasers
Molecular
Optical and Plasma Physics
Photoelectric emission
Photoelectrons
Photons
Physical Chemistry
Physics
Physics and Astronomy
Polarization
Quantum Information Technology
Quantum numbers
Quantum Physics
Regular Article – Ultraintense and Ultrashort Laser Fields
Schrodinger equation
Spectroscopy/Spectrometry
Spintronics
title Linear dichroism in few-photon ionization of laser-dressed helium
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