Linear dichroism in few-photon ionization of laser-dressed helium
Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay betw...
Gespeichert in:
Veröffentlicht in: | The European physical journal. D, Atomic, molecular, and optical physics Atomic, molecular, and optical physics, 2021-07, Vol.75 (7), Article 205 |
---|---|
Hauptverfasser: | , , , , , , , , , , , , , , |
Format: | Artikel |
Sprache: | eng |
Schlagworte: | |
Online-Zugang: | Volltext |
Tags: |
Tag hinzufügen
Keine Tags, Fügen Sie den ersten Tag hinzu!
|
container_end_page | |
---|---|
container_issue | 7 |
container_start_page | |
container_title | The European physical journal. D, Atomic, molecular, and optical physics |
container_volume | 75 |
creator | Meister, Severin Bondy, Aaron Schnorr, Kirsten Augustin, Sven Lindenblatt, Hannes Trost, Florian Xie, Xinhua Braune, Markus Manschwetus, Bastian Schirmel, Nora Redlin, Harald Douguet, Nicolas Pfeifer, Thomas Bartschat, Klaus Moshammer, Robert |
description | Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation.
Graphic abstract |
doi_str_mv | 10.1140/epjd/s10053-021-00218-0 |
format | Article |
fullrecord | <record><control><sourceid>proquest_cross</sourceid><recordid>TN_cdi_proquest_journals_2552288795</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>2552288795</sourcerecordid><originalsourceid>FETCH-LOGICAL-c329t-7d11bb066e7c2cce61da83b6fa8498cb5e78ad6c02a4a1f739efb10ad6c4f7513</originalsourceid><addsrcrecordid>eNqFkE9LxDAQxYMouK5-Bgueo5O0TdLjsvgPFrzoOaTpxM2y29Ski-inN2tFj17mDcN7b-BHyCWDa8YquMFh090kBlCXFDijkIeicERmrCorKkA2x7-7gFNyltIGsquuxIwsVr5HE4vO23UMPu0K3xcO3-mwDmPoCx96_2nGLEVwxdYkjLSLmBJ2xRq3fr87JyfObBNe_OicvNzdPi8f6Orp_nG5WFFb8maksmOsbUEIlJZbi4J1RpWtcEZVjbJtjVKZTljgpjLMybJB1zI4nCona1bOydXUO8Twtsc06k3Yxz6_1LyuOVdKNnV2ycllY0gpotND9DsTPzQDfeClD7z0xEtnVPqbl4acVFMy5UT_ivGv_7_oF1SXchA</addsrcrecordid><sourcetype>Aggregation Database</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>2552288795</pqid></control><display><type>article</type><title>Linear dichroism in few-photon ionization of laser-dressed helium</title><source>SpringerLink Journals - AutoHoldings</source><creator>Meister, Severin ; Bondy, Aaron ; Schnorr, Kirsten ; Augustin, Sven ; Lindenblatt, Hannes ; Trost, Florian ; Xie, Xinhua ; Braune, Markus ; Manschwetus, Bastian ; Schirmel, Nora ; Redlin, Harald ; Douguet, Nicolas ; Pfeifer, Thomas ; Bartschat, Klaus ; Moshammer, Robert</creator><creatorcontrib>Meister, Severin ; Bondy, Aaron ; Schnorr, Kirsten ; Augustin, Sven ; Lindenblatt, Hannes ; Trost, Florian ; Xie, Xinhua ; Braune, Markus ; Manschwetus, Bastian ; Schirmel, Nora ; Redlin, Harald ; Douguet, Nicolas ; Pfeifer, Thomas ; Bartschat, Klaus ; Moshammer, Robert</creatorcontrib><description>Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation.
Graphic abstract</description><identifier>ISSN: 1434-6060</identifier><identifier>EISSN: 1434-6079</identifier><identifier>DOI: 10.1140/epjd/s10053-021-00218-0</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Applications of Nonlinear Dynamics and Chaos Theory ; Atomic ; Dichroism ; Excitation ; Helium ; Infrared radiation ; Ionization ; Lasers ; Molecular ; Optical and Plasma Physics ; Photoelectric emission ; Photoelectrons ; Photons ; Physical Chemistry ; Physics ; Physics and Astronomy ; Polarization ; Quantum Information Technology ; Quantum numbers ; Quantum Physics ; Regular Article – Ultraintense and Ultrashort Laser Fields ; Schrodinger equation ; Spectroscopy/Spectrometry ; Spintronics</subject><ispartof>The European physical journal. D, Atomic, molecular, and optical physics, 2021-07, Vol.75 (7), Article 205</ispartof><rights>The Author(s) 2021</rights><rights>The Author(s) 2021. This work is published under http://creativecommons.org/licenses/by/4.0/ (the “License”). Notwithstanding the ProQuest Terms and Conditions, you may use this content in accordance with the terms of the License.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c329t-7d11bb066e7c2cce61da83b6fa8498cb5e78ad6c02a4a1f739efb10ad6c4f7513</cites><orcidid>0000-0002-5245-8377</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://link.springer.com/content/pdf/10.1140/epjd/s10053-021-00218-0$$EPDF$$P50$$Gspringer$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://link.springer.com/10.1140/epjd/s10053-021-00218-0$$EHTML$$P50$$Gspringer$$Hfree_for_read</linktohtml><link.rule.ids>314,780,784,27924,27925,41488,42557,51319</link.rule.ids></links><search><creatorcontrib>Meister, Severin</creatorcontrib><creatorcontrib>Bondy, Aaron</creatorcontrib><creatorcontrib>Schnorr, Kirsten</creatorcontrib><creatorcontrib>Augustin, Sven</creatorcontrib><creatorcontrib>Lindenblatt, Hannes</creatorcontrib><creatorcontrib>Trost, Florian</creatorcontrib><creatorcontrib>Xie, Xinhua</creatorcontrib><creatorcontrib>Braune, Markus</creatorcontrib><creatorcontrib>Manschwetus, Bastian</creatorcontrib><creatorcontrib>Schirmel, Nora</creatorcontrib><creatorcontrib>Redlin, Harald</creatorcontrib><creatorcontrib>Douguet, Nicolas</creatorcontrib><creatorcontrib>Pfeifer, Thomas</creatorcontrib><creatorcontrib>Bartschat, Klaus</creatorcontrib><creatorcontrib>Moshammer, Robert</creatorcontrib><title>Linear dichroism in few-photon ionization of laser-dressed helium</title><title>The European physical journal. D, Atomic, molecular, and optical physics</title><addtitle>Eur. Phys. J. D</addtitle><description>Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation.
Graphic abstract</description><subject>Applications of Nonlinear Dynamics and Chaos Theory</subject><subject>Atomic</subject><subject>Dichroism</subject><subject>Excitation</subject><subject>Helium</subject><subject>Infrared radiation</subject><subject>Ionization</subject><subject>Lasers</subject><subject>Molecular</subject><subject>Optical and Plasma Physics</subject><subject>Photoelectric emission</subject><subject>Photoelectrons</subject><subject>Photons</subject><subject>Physical Chemistry</subject><subject>Physics</subject><subject>Physics and Astronomy</subject><subject>Polarization</subject><subject>Quantum Information Technology</subject><subject>Quantum numbers</subject><subject>Quantum Physics</subject><subject>Regular Article – Ultraintense and Ultrashort Laser Fields</subject><subject>Schrodinger equation</subject><subject>Spectroscopy/Spectrometry</subject><subject>Spintronics</subject><issn>1434-6060</issn><issn>1434-6079</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2021</creationdate><recordtype>article</recordtype><sourceid>C6C</sourceid><recordid>eNqFkE9LxDAQxYMouK5-Bgueo5O0TdLjsvgPFrzoOaTpxM2y29Ski-inN2tFj17mDcN7b-BHyCWDa8YquMFh090kBlCXFDijkIeicERmrCorKkA2x7-7gFNyltIGsquuxIwsVr5HE4vO23UMPu0K3xcO3-mwDmPoCx96_2nGLEVwxdYkjLSLmBJ2xRq3fr87JyfObBNe_OicvNzdPi8f6Orp_nG5WFFb8maksmOsbUEIlJZbi4J1RpWtcEZVjbJtjVKZTljgpjLMybJB1zI4nCona1bOydXUO8Twtsc06k3Yxz6_1LyuOVdKNnV2ycllY0gpotND9DsTPzQDfeClD7z0xEtnVPqbl4acVFMy5UT_ivGv_7_oF1SXchA</recordid><startdate>20210701</startdate><enddate>20210701</enddate><creator>Meister, Severin</creator><creator>Bondy, Aaron</creator><creator>Schnorr, Kirsten</creator><creator>Augustin, Sven</creator><creator>Lindenblatt, Hannes</creator><creator>Trost, Florian</creator><creator>Xie, Xinhua</creator><creator>Braune, Markus</creator><creator>Manschwetus, Bastian</creator><creator>Schirmel, Nora</creator><creator>Redlin, Harald</creator><creator>Douguet, Nicolas</creator><creator>Pfeifer, Thomas</creator><creator>Bartschat, Klaus</creator><creator>Moshammer, Robert</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>C6C</scope><scope>AAYXX</scope><scope>CITATION</scope><orcidid>https://orcid.org/0000-0002-5245-8377</orcidid></search><sort><creationdate>20210701</creationdate><title>Linear dichroism in few-photon ionization of laser-dressed helium</title><author>Meister, Severin ; Bondy, Aaron ; Schnorr, Kirsten ; Augustin, Sven ; Lindenblatt, Hannes ; Trost, Florian ; Xie, Xinhua ; Braune, Markus ; Manschwetus, Bastian ; Schirmel, Nora ; Redlin, Harald ; Douguet, Nicolas ; Pfeifer, Thomas ; Bartschat, Klaus ; Moshammer, Robert</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c329t-7d11bb066e7c2cce61da83b6fa8498cb5e78ad6c02a4a1f739efb10ad6c4f7513</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Applications of Nonlinear Dynamics and Chaos Theory</topic><topic>Atomic</topic><topic>Dichroism</topic><topic>Excitation</topic><topic>Helium</topic><topic>Infrared radiation</topic><topic>Ionization</topic><topic>Lasers</topic><topic>Molecular</topic><topic>Optical and Plasma Physics</topic><topic>Photoelectric emission</topic><topic>Photoelectrons</topic><topic>Photons</topic><topic>Physical Chemistry</topic><topic>Physics</topic><topic>Physics and Astronomy</topic><topic>Polarization</topic><topic>Quantum Information Technology</topic><topic>Quantum numbers</topic><topic>Quantum Physics</topic><topic>Regular Article – Ultraintense and Ultrashort Laser Fields</topic><topic>Schrodinger equation</topic><topic>Spectroscopy/Spectrometry</topic><topic>Spintronics</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Meister, Severin</creatorcontrib><creatorcontrib>Bondy, Aaron</creatorcontrib><creatorcontrib>Schnorr, Kirsten</creatorcontrib><creatorcontrib>Augustin, Sven</creatorcontrib><creatorcontrib>Lindenblatt, Hannes</creatorcontrib><creatorcontrib>Trost, Florian</creatorcontrib><creatorcontrib>Xie, Xinhua</creatorcontrib><creatorcontrib>Braune, Markus</creatorcontrib><creatorcontrib>Manschwetus, Bastian</creatorcontrib><creatorcontrib>Schirmel, Nora</creatorcontrib><creatorcontrib>Redlin, Harald</creatorcontrib><creatorcontrib>Douguet, Nicolas</creatorcontrib><creatorcontrib>Pfeifer, Thomas</creatorcontrib><creatorcontrib>Bartschat, Klaus</creatorcontrib><creatorcontrib>Moshammer, Robert</creatorcontrib><collection>Springer Nature OA Free Journals</collection><collection>CrossRef</collection><jtitle>The European physical journal. D, Atomic, molecular, and optical physics</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Meister, Severin</au><au>Bondy, Aaron</au><au>Schnorr, Kirsten</au><au>Augustin, Sven</au><au>Lindenblatt, Hannes</au><au>Trost, Florian</au><au>Xie, Xinhua</au><au>Braune, Markus</au><au>Manschwetus, Bastian</au><au>Schirmel, Nora</au><au>Redlin, Harald</au><au>Douguet, Nicolas</au><au>Pfeifer, Thomas</au><au>Bartschat, Klaus</au><au>Moshammer, Robert</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Linear dichroism in few-photon ionization of laser-dressed helium</atitle><jtitle>The European physical journal. D, Atomic, molecular, and optical physics</jtitle><stitle>Eur. Phys. J. D</stitle><date>2021-07-01</date><risdate>2021</risdate><volume>75</volume><issue>7</issue><artnum>205</artnum><issn>1434-6060</issn><eissn>1434-6079</eissn><abstract>Ionization of laser-dressed atomic helium is investigated with focus on photoelectron angular distributions stemming from two-color multi-photon excited states. The experiment combines extreme ultraviolet (XUV) with infrared (IR) radiation, while the relative polarization and the temporal delay between the pulses can be varied. By means of an XUV photon energy scan over several electronvolts, we get access to excited states in the dressed atom exhibiting various binding energies, angular momenta, and magnetic quantum numbers. Furthermore, varying the relative polarization is employed as a handle to switch on and off the population of certain states that are only accessible by two-photon excitation. In this way, photoemission can be suppressed for specific XUV photon energies. Additionally, we investigate the dependence of the photoelectron angular distributions on the IR laser intensity. At our higher IR intensities, we start leaving the simple multi-photon ionization regime. The interpretation of the experimental results is supported by numerically solving the time-dependent Schrödinger equation in a single-active-electron approximation.
Graphic abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><doi>10.1140/epjd/s10053-021-00218-0</doi><orcidid>https://orcid.org/0000-0002-5245-8377</orcidid><oa>free_for_read</oa></addata></record> |
fulltext | fulltext |
identifier | ISSN: 1434-6060 |
ispartof | The European physical journal. D, Atomic, molecular, and optical physics, 2021-07, Vol.75 (7), Article 205 |
issn | 1434-6060 1434-6079 |
language | eng |
recordid | cdi_proquest_journals_2552288795 |
source | SpringerLink Journals - AutoHoldings |
subjects | Applications of Nonlinear Dynamics and Chaos Theory Atomic Dichroism Excitation Helium Infrared radiation Ionization Lasers Molecular Optical and Plasma Physics Photoelectric emission Photoelectrons Photons Physical Chemistry Physics Physics and Astronomy Polarization Quantum Information Technology Quantum numbers Quantum Physics Regular Article – Ultraintense and Ultrashort Laser Fields Schrodinger equation Spectroscopy/Spectrometry Spintronics |
title | Linear dichroism in few-photon ionization of laser-dressed helium |
url | https://sfx.bib-bvb.de/sfx_tum?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-01-06T16%3A43%3A37IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_cross&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Linear%20dichroism%20in%20few-photon%20ionization%20of%20laser-dressed%20helium&rft.jtitle=The%20European%20physical%20journal.%20D,%20Atomic,%20molecular,%20and%20optical%20physics&rft.au=Meister,%20Severin&rft.date=2021-07-01&rft.volume=75&rft.issue=7&rft.artnum=205&rft.issn=1434-6060&rft.eissn=1434-6079&rft_id=info:doi/10.1140/epjd/s10053-021-00218-0&rft_dat=%3Cproquest_cross%3E2552288795%3C/proquest_cross%3E%3Curl%3E%3C/url%3E&disable_directlink=true&sfx.directlink=off&sfx.report_link=0&rft_id=info:oai/&rft_pqid=2552288795&rft_id=info:pmid/&rfr_iscdi=true |