Indirect coal liquefaction by integrated entrained flow gasification and Rectisol/Fischer–Tropsch processes for producing automobile diesel substitutes
Herein, we describe the design and operation of an indirect coal liquefaction plant with integrated coal-water slurry manufacturing, entrained flow gasification, Rectisol, and Fischer–Tropsch processes to produce liquid fuels for vehicles. The above plant contained an entrained flow gasifier (10 t/d...
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Veröffentlicht in: | Energy (Oxford) 2021-03, Vol.219, p.119597, Article 119597 |
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Sprache: | eng |
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Zusammenfassung: | Herein, we describe the design and operation of an indirect coal liquefaction plant with integrated coal-water slurry manufacturing, entrained flow gasification, Rectisol, and Fischer–Tropsch processes to produce liquid fuels for vehicles. The above plant contained an entrained flow gasifier (10 t/d test rig) operated using oxygen as a gasifying agent (21 bar, 1100 °C) and could stably produce synthesis gas (37.8 vol% H2, 36.4 vol% CO) at 600 Nm3/h. Due to the importance of impurities in synthetic liquid fuel production, more than 99% of H2S contained in synthesis gas was removed by the Rectisol process employing refrigerated methanol. An iron-based catalyst allowed liquid fuels containing wax, light/heavy oil, and alcohol fractions to be obtained by the Fischer–Tropsch process at a rate of 5 barrel per day, with detailed analysis confirming their compliance with various quality standards and thus their suitability for use as automobile diesel after distillation.
•Integrated entrained flow gasifier and Rectisol/Fisher-Tropsch process was described.•The synthesis gas (37.8 vol% H2, 36.4 vol% CO) at 600 Nm3/h was produced.•More than 99% of H2S contained in synthesis gas was removed in Rectisol process.•The liquid fuels can be successfully produced by pilot-scale F-T synthesis.•Distilled ICTL diesel can be a viable alternative for the commercial diesel. |
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ISSN: | 0360-5442 1873-6785 |
DOI: | 10.1016/j.energy.2020.119597 |