A QCL-based metrological-grade source at 6 μm

In view of high-precision molecular spectroscopy in the infrared, we realized a narrow-linewidth laser source at 5.8 μ m traceable to the second in the International System of Units by mixing two near-infrared lasers in an orientation-patterned GaP crystal. The generated radiation is traceable to a Cs fountain through an optical fiber-delivered carrier; its estimated linewidth is 2.3 kHz at 1 s integration time. A quantum cascade laser emitting at the same wavelength is used to boost the power of the mid-IR radiation up to few tens of mW. Thanks to a phase-locking loop, about 70% of the quantum cascade laser output power is within the linewidth of the difference-frequency radiation. This apparatus is used for absolute molecular spectroscopy in a region, above 5 μ m, where high-precision traceability and reliable operation are still challenging. In this paper, we provide the basic information to implement a powerful and metrological grade source in the mid-infrared for precision measurements.