Frontispiece: Catalytic Ammonia Oxidation to Dinitrogen by Hydrogen Atom Abstraction

Frontispiece: Catalytic Ammonia Oxidation to Dinitrogen by Hydrogen Atom Abstraction

Ammonia Oxidation A molecular Ru‐based catalyst converts NH3 into N2, as reported by M. T. Mock et al. in their Communication on page 11618. The cleavage of six N−H bonds was achieved by coupling H+ and e− transfers using the tBu3ArO. radical as the H atom acceptor.

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Veröffentlicht in:Angewandte Chemie International Edition 2019-08, Vol.58 (34), p.n/a
Hauptverfasser: Bhattacharya, Papri, Heiden, Zachariah M., Chambers, Geoffrey M., Johnson, Samantha I., Bullock, R. Morris, Mock, Michael T.
Format: Artikel
Sprache:eng
Schlagworte:
Ammonia
ammonia oxidation
Catalysis
Catalysts
Coupling (molecular)
dinitrogen
homogeneous catalysis
Hydrogen
Oxidation
radical reactions
ruthenium
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Zusammenfassung:Ammonia Oxidation A molecular Ru‐based catalyst converts NH3 into N2, as reported by M. T. Mock et al. in their Communication on page 11618. The cleavage of six N−H bonds was achieved by coupling H+ and e− transfers using the tBu3ArO. radical as the H atom acceptor.
ISSN:1433-7851
1521-3773
DOI:10.1002/anie.201983461