The influence of the incommensurately modulated structure on the physical properties of Fe1.35Ge

Single crystal growth by chemical vapour transport has resulted samples with Fe1.35Ge stoichiometry. Structural study has shown that the large number of vacancies introduces an incommensuately modulated structure. The electrical resistivity is in the 200 μΩcm range at room temperature, and although the ferromagnetic transition temperature at 425 K is clearly visible, it hardly varies down to 4.2 K. It is suggested that the large number of vacancies (and the incommensurate modulation) introduce a strong backscattering, and the system is at the brink of a Mooij correlation. The thermal conductivity and Seebeck coefficient carry also the consequences of the high concentration of vacancies. •We report incommensuately modulated structure in Fe1.35Ge phase.•Electrical resistivity has very weak temperature dependence in Fe1.35Ge phase.•Fe1.35Ge phase exhibits soft magnetic properties.