Multi-color fluorescent carbon dots with single wavelength excitation for white light-emitting diodes

Carbon dots (CDs) have been applied in numerous fields by virtue of their excellent features. Multi-color fluorescent carbon dots with high photoluminescence (PL) quantum yield are still the emphases for research. Here, by using 3,5-diaminobenzoic acid and 3,4-diaminobenzoic acid, multi-color-red, g...

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Veröffentlicht in:Journal of alloys and compounds 2019-07, Vol.793, p.613-619
Hauptverfasser: Zhao, Kangxu, Zheng, Xuan, Zhang, Huijun, Xu, Menghan, Wang, Shan, Yang, Quanling, Xiong, Chuanxi
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Sprache:eng
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Zusammenfassung:Carbon dots (CDs) have been applied in numerous fields by virtue of their excellent features. Multi-color fluorescent carbon dots with high photoluminescence (PL) quantum yield are still the emphases for research. Here, by using 3,5-diaminobenzoic acid and 3,4-diaminobenzoic acid, multi-color-red, green, blue (RGB) emitting CDs (RGB-CDs) were successfully synthesized via a one-pot solvothermal route. The RGB-CDs exhibited stable optical properties and significant photoluminescence characteristics with excitation-independent. Structure and element analysis indicated that conjugated graphite structure of carbon cores and oxygen on surface states were responsible for the RGB color emissions of carbon dots. Moreover, RGB-color and white light-emitting diodes (LEDs) were fabricated by these multi-color fluorescent carbon dots. The LEDs exhibited excellent lighting performance, indicating that these RGB-CDs have the potential to substitute rare elements for solid-state optoelectronic applications. [Display omitted] •Carbon dots (CDs) with blue, green, and red fluorescence emissions were synthesized.•RGB-CDs/PDMS films exhibited high photoluminescence stability.•CDs-based LEDs with trichromatic luminescence as well as white light were successfully fabricated.
ISSN:0925-8388
1873-4669
DOI:10.1016/j.jallcom.2019.04.146