Magnetic field induced evolution of highly resistant Griffiths phase in fine grain manganite La0.75Ca0.25MnO3

•Griffiths like phase is detected between 232 and 280 K in mixed valence manganite La0.75Ca0.25MnO3.•Griffiths like phase persists up to 3000 Oe.•Griffiths phase magnetization decays with rising temperature. The Griffiths phase in fine grain manganite La0.75Ca0.25MnO3 is studied by the complementary...

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Veröffentlicht in:Journal of magnetism and magnetic materials 2019-04, Vol.475, p.189-194
Hauptverfasser: Pękała, M., Pękała, K., Szydłowska, J., Drozd, V.
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Sprache:eng
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Zusammenfassung:•Griffiths like phase is detected between 232 and 280 K in mixed valence manganite La0.75Ca0.25MnO3.•Griffiths like phase persists up to 3000 Oe.•Griffiths phase magnetization decays with rising temperature. The Griffiths phase in fine grain manganite La0.75Ca0.25MnO3 is studied by the complementary structural methods, DC magnetic susceptibility and ESR spectroscopy. The Griffiths like phase is detected above Curie temperature between 232 and 280 K and sustains up to high magnetic field of 3000 Oe. The magnetic susceptibility of Griffiths phase is a decreasing function of temperature. The magnetic field dependence of Griffiths phase susceptibility reveals its remarkable contribution to measured total susceptibility. The additional anomalous ESR signal supperimpossed on the paramagnetic one is ascribed to the locally inhomogeneous Griffiths like phase in agreement with the core – shell model.
ISSN:0304-8853
1873-4766
DOI:10.1016/j.jmmm.2018.11.069