Self-biased large magnetoelectric coupling in co-sintered Bi0.5Na0.5TiO3 based piezoelectric and CoFe2O4 based magnetostrictive bilayered composite

In this work, magnetoelectric properties of a co-sintered bilayered composite of non-lead based piezoelectric 0.97(Bi0.5Na0.5TiO3)–0.03(K0.47Na0.47Li0.06Nb0.74Sb0.06Ta0.2O3) and magnetostrictive Co0.6Zn0.4Fe1.7Mn0.3O4 are presented. Similar optimal sintering conditions of the individual components l...

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Veröffentlicht in:Journal of applied physics 2014-12, Vol.116 (24)
Hauptverfasser: Kumari, Mukesh, Singh, Amrita, Gupta, Arti, Prakash, Chandra, Chatterjee, Ratnamala
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Sprache:eng
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Zusammenfassung:In this work, magnetoelectric properties of a co-sintered bilayered composite of non-lead based piezoelectric 0.97(Bi0.5Na0.5TiO3)–0.03(K0.47Na0.47Li0.06Nb0.74Sb0.06Ta0.2O3) and magnetostrictive Co0.6Zn0.4Fe1.7Mn0.3O4 are presented. Similar optimal sintering conditions of the individual components lead to a very clean interface as evidenced in the scanning electron microscopy, angle dispersive X-ray diffraction, and energy-dispersive X-ray (EDX) results. Clean interface results in strong intimate mechanical coupling between both components and causes a maximum transfer of induced strain, leading to a large magnetoelectric coupling ∼142 mV/cm·Oe measured in longitudinally magnetized-transversely polarized configuration (L-T mode). Remnant polarization ∼32 μC/cm2, remnant magnetization ∼0.50 emu/g, and sufficiently high self biased magnetoelectricity ∼135 mV/cm Oe (L-T mode) were observed for this composite.
ISSN:0021-8979
1089-7550
DOI:10.1063/1.4904758