Ionic Skin with Biomimetic Dielectric Layer Templated from Calathea Zebrine Leaf

Flexible electronic skins (e‐skins) with high sensitivity and broad‐range pressure sensing are highly desired in artificial intelligence, and human–machine interaction. Capacitive‐type e‐skins have a simple configuration, but the change in dimensions of the dielectric layer is often quite limited, although introducing surface microstructures might improve the sensitivity in some extent. Moreover, such surface structures typically require costly microfabrication methods to fabricate. Here, a low‐cost microstructured ionic gel (MIG) with uniform cone‐like surface microstructures for high‐performance capacitive e‐skins is reported. The MIG film is templated from a Calathea zebrine leaf using soft lithography, and sandwiched by two flexible electrodes. The device exhibits a low limit of detection down to 0.1 Pa, a ultrahigh sensitivity of 54.31 kPa−1 in the low pressure regime (