Enhancement and stabilization of plasma using collinear long-short double-pulse laser-induced breakdown spectroscopy

A collinear long-short dual-pulse laser-induced breakdown spectroscopy (DP-LIBS) method was employed to enhance and stabilize the laser-induced plasma from steel sample. The long-pulse-width laser beam with the pulse width of 60μs was generated by a Nd: YAG laser which was operated at FR (free running) mode. The comparative experiments were carried out between single pulse LIBS (SP-LIBS) and long-short DP-LIBS. The recorded results showed that the emission intensities and the temperature of plasma were enhanced by long-short DP-LIBS. The plasma images showed that the plasma was bigger and had a longer lifetime in long-short DP-LIBS situation. Through the calculation of time-resolved plasma temperature and intensity ratio, it can be concluded that the plasma was stabilized by the long-pulse-width laser beam. The long-short DP-LIBS method also generated the stable plasma condition from the samples with different initial temperatures, which overcame the difficulties of LIBS in the online measurement for steel production line. [Display omitted] •A long-short DP-LIBS method was employed to enhance and stabilize the laser-induced plasma.•Compared with SP-LIBS, the plasma was bigger and had a longer lifetime in long-short DP-LIBS condition.•The plasma was maintained at a stable and high temperature using long-short DP-LIBS.•The measured spectra by long-short DP-LIBS showed a conformity at different initial temperatures of the sample.